Nanomotors driven by single-atom catalysts

被引:7
|
作者
Chen, Shuai [2 ]
Wang, Jianhong [3 ]
Cao, Shoupeng [2 ]
Al-Hilfi, Samir H. [2 ]
Yang, Juan [1 ]
Bonn, Mischa [2 ]
van Hest, Jan C. M. [3 ]
Shao, Jingxin [3 ]
Mullen, Klaus [2 ]
Zhou, Yazhou [1 ,2 ]
机构
[1] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang 212013, Jiangsu, Peoples R China
[2] Max Planck Inst Polymer Res, D-55128 Mainz, Germany
[3] Eindhoven Univ Technol, Inst Complex Mol Syst, Bioorgan Chem, NL-5600 MB Eindhoven, Netherlands
来源
CELL REPORTS PHYSICAL SCIENCE | 2024年 / 5卷 / 04期
基金
欧洲研究理事会;
关键词
FABRICATION;
D O I
10.1016/j.xcrp.2024.101898
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Single -atom catalysts (SACs) involve atomically dispersed metal atoms on solid supports. SACs combine the fast reaction kinetics of homogeneous catalysts with the recyclability of heterogeneous catalysts, providing great technological opportunities. To date, SAC research has focused primarily on the development of synthetic methods and fuel production. Here, we report a combination of SAC and nanomotor design to fabricate motile systems, referred to here as SAC-nanomotors. This concept is demonstrated by an Fe SAC prepared via the pulsing H 2 -pyrolysis approach. The Fe SAC -nanomotor is powered by decomposing H 2 O 2 with ultrahigh -density Fe atoms, achieving a velocity of 18 G 3 mm s - 1 at a low fuel concentration of 10 mM. This proof -of -principle SAC-nanomotor, with the smallest possible catalytic combustion site and excellent biocompatibility, illustrates the enormous potential of SACs for developing advanced nanomotor systems.
引用
收藏
页数:14
相关论文
共 50 条
  • [41] Recent progresses in the research of single-atom catalysts
    Jun Li
    Yadong Li
    Tao Zhang
    Science China Materials, 2020, 63 : 889 - 891
  • [42] Construction and application of Pt single-atom catalysts
    Zhang, Min
    Wei, Juanjuan
    Ouyang, Jin
    Na, Na
    Chinese Journal of Analysis Laboratory, 2022, 41 (12) : 1400 - 1410
  • [43] Progress in electrocatalysis by single-atom site catalysts
    Zhu T.
    Han Y.
    Liu S.
    Xie W.
    Yuan B.
    Song H.
    Chegn F.
    Huagong Jinzhan/Chemical Industry and Engineering Progress, 2022, 41 (02): : 666 - 681
  • [44] Local structural environment of single-atom catalysts
    Chen, Zheng
    Han, Lili
    INORGANIC CHEMISTRY FRONTIERS, 2023, 11 (01) : 29 - 49
  • [45] The Multifaceted Reactivity of Single-Atom Heterogeneous Catalysts
    Mitchell, Sharon
    Vorobyeva, Evgeniya
    Perez-Ramirez, Javier
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2018, 57 (47) : 15316 - 15329
  • [46] Robust single-atom catalysts for better catalysis
    Liu, Jingyue
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2019, 258
  • [47] Advances in single-atom catalysts for oxygen electrodes
    Wang Y.
    Tang Y.
    Huagong Xuebao/CIESC Journal, 2020, 71 (10): : 4409 - 4428
  • [48] Single-atom catalysts: The role of intrinsic intermediate
    Li, Yafei
    GREEN ENERGY & ENVIRONMENT, 2020, 5 (01) : 4 - 5
  • [49] Recent progresses in the research of single-atom catalysts
    Li, Jun
    Li, Yadong
    Zhang, Tao
    SCIENCE CHINA-MATERIALS, 2020, 63 (06) : 889 - 891
  • [50] Single-atom iron catalysts for biomedical applications
    Tang, Jing
    Wu, Yifan
    Li, Xun
    Bu, Lihong
    Chang, Baisong
    PROGRESS IN MATERIALS SCIENCE, 2022, 128