Nanomotors driven by single-atom catalysts

被引:7
|
作者
Chen, Shuai [2 ]
Wang, Jianhong [3 ]
Cao, Shoupeng [2 ]
Al-Hilfi, Samir H. [2 ]
Yang, Juan [1 ]
Bonn, Mischa [2 ]
van Hest, Jan C. M. [3 ]
Shao, Jingxin [3 ]
Mullen, Klaus [2 ]
Zhou, Yazhou [1 ,2 ]
机构
[1] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang 212013, Jiangsu, Peoples R China
[2] Max Planck Inst Polymer Res, D-55128 Mainz, Germany
[3] Eindhoven Univ Technol, Inst Complex Mol Syst, Bioorgan Chem, NL-5600 MB Eindhoven, Netherlands
来源
CELL REPORTS PHYSICAL SCIENCE | 2024年 / 5卷 / 04期
基金
欧洲研究理事会;
关键词
FABRICATION;
D O I
10.1016/j.xcrp.2024.101898
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Single -atom catalysts (SACs) involve atomically dispersed metal atoms on solid supports. SACs combine the fast reaction kinetics of homogeneous catalysts with the recyclability of heterogeneous catalysts, providing great technological opportunities. To date, SAC research has focused primarily on the development of synthetic methods and fuel production. Here, we report a combination of SAC and nanomotor design to fabricate motile systems, referred to here as SAC-nanomotors. This concept is demonstrated by an Fe SAC prepared via the pulsing H 2 -pyrolysis approach. The Fe SAC -nanomotor is powered by decomposing H 2 O 2 with ultrahigh -density Fe atoms, achieving a velocity of 18 G 3 mm s - 1 at a low fuel concentration of 10 mM. This proof -of -principle SAC-nanomotor, with the smallest possible catalytic combustion site and excellent biocompatibility, illustrates the enormous potential of SACs for developing advanced nanomotor systems.
引用
收藏
页数:14
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