Prompt Charge Separation at Crystalline-Amorphous Interfaces of Poly(heptazine imides) for Photocatalytic Hydrogen Evolution

被引:4
|
作者
Wang, Qian [1 ]
Li, Shiyao [1 ]
Zheng, Dandan [1 ]
Wang, Sibo [1 ]
Hou, Yidong [1 ]
Zhang, Guigang [1 ]
机构
[1] Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350108, Peoples R China
来源
ACS APPLIED ENERGY MATERIALS | 2024年 / 7卷 / 15期
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
charge separation; photocatalysis; poly(heptazineimide); hydrogen production; water splitting; CARBON NITRIDE; WATER;
D O I
10.1021/acsaem.4c01512
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The development of effective, low-cost, and stable photocatalysts for visible-light-driven hydrogen production is desired but challenging. Herein, in the presence of a ternary eutectic salt mixture, poly(heptazine imide) with a crystalline-amorphous interface, is synthesized, which endows improved transfer of charge carriers and enhanced photocatalytic activity for hydrogen production.
引用
收藏
页码:6090 / 6095
页数:6
相关论文
共 50 条
  • [41] Crystalline-amorphous M@MNx (M = Co, Fe, Ni) encapsulated in nitrogen-doped carbon for enhanced efficient and durable hydrogen evolution reaction
    Yang, Yang
    Duan, Xiao-Chuan
    Guo, Shao-Hui
    Zhang, Xian-Ming
    RARE METALS, 2024, 43 (04) : 1547 - 1556
  • [42] Constructing crystalline/amorphous interfaces in crystalline vanadium disulfide/amorphous molybdenum sulfide/reduced graphene oxide nanocomposites via a hydrothermal-plasma method toward efficient hydrogen evolution reaction
    Zhang, Dai
    Chen, Yuanyuan
    Dai, Hanqing
    Lv, Xuewei
    Guo, Ruiqian
    Ou, Qiongrong
    Zhang, Shuyu
    CATALYSIS TODAY, 2023, 422
  • [43] Preparation of highly crystalline quaternary heterostructure catalyst for hydrogen evolution under solar light: Improved photoexcited charge separation
    Mandari, Kotesh Kumar
    Do, Jeong Yeon
    Pandey, Sadanand
    Vattikuti, S. V. Prabhakar
    Kang, Misook
    MATERIALS RESEARCH BULLETIN, 2020, 122
  • [44] Controllable phase transition dependent photoinduced charge separation in CuFe2O4 for photocatalytic hydrogen evolution
    Hou, Dongfen
    Tian, Jingqi
    Wei, Jingying
    Jia, Dailing
    Ma, Ke
    Xue, Huaiguo
    Jiang, Tengfei
    INORGANIC CHEMISTRY FRONTIERS, 2024, 11 (15): : 4846 - 4854
  • [45] Surface Engineering for Extremely Enhanced Charge Separation and Photocatalytic Hydrogen Evolution on g-C3N4
    Yu, Yu
    Yan, Wei
    Wang, Xiaofang
    Li, Pei
    Gao, Wenyu
    Zou, Haihan
    Wu, Songmei
    Ding, Kejian
    ADVANCED MATERIALS, 2018, 30 (09)
  • [46] Dipole polarization-driven spatial charge separation in defective zinc cadmium sulfoselenide for boosting photocatalytic hydrogen evolution
    Tian, Qingzheng
    Wang, Li
    Sun, Weiwei
    Meng, Alan
    Yang, Lina
    Li, Zhenjiang
    APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY, 2024, 359
  • [47] Carbon Quantum Dot Implanted Graphite Carbon Nitride Nanotubes: Excellent Charge Separation and Enhanced Photocatalytic Hydrogen Evolution
    Wang, Yang
    Liu, Xueqin
    Liu, Jia
    Han, Bo
    Hu, Xiaoqin
    Yang, Fan
    Xu, Zuwei
    Li, Yinchang
    Jia, Songru
    Li, Zhen
    Zhao, Yanli
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2018, 57 (20) : 5765 - 5771
  • [48] Simultaneous formation of mesopores and homojunctions in graphite carbon nitride with enhanced optical absorption, charge separation and photocatalytic hydrogen evolution
    Ba, Guiming
    Liang, Zhiwei
    Li, Haiping
    Du, Na
    Liu, Jianqiang
    Hou, Wanguo
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 253 : 359 - 368
  • [49] Understanding charge separation in CdS/Ce-UiO66-NH2 heterojunctions for enhanced photocatalytic hydrogen evolution
    Hou, Wenqing
    Hillman, Sam A. J.
    Gonzalez-Carrero, Soranyel
    Yao, Shilin
    Zhu, Huangtianzhi
    Durrant, James R.
    SUSTAINABLE ENERGY & FUELS, 2025, 9 (02): : 576 - 584
  • [50] Rational construction of multiple interfaces in ternary heterostructure for efficient spatial separation and transfer of photogenerated carriers in the application of photocatalytic hydrogen evolution
    Shi, Jian-Wen
    Ma, Dandan
    Zou, Yajun
    Fan, Zhaoyang
    Shi, Jinwen
    Cheng, Linhao
    Ji, Xin
    Niu, Chunming
    JOURNAL OF POWER SOURCES, 2018, 379 : 249 - 260