Recent advances in dynamic reconstruction of electrocatalysts for carbon dioxide reduction

被引：4

作者：

Zhang, Jianfang ^{[1
,2
]}

Xia, Shuai ^{[1
]}

Wang, Yan ^{[1
,3
]}

Wu, Jingjie ^{[2
]}

Wu, Yucheng ^{[1
,4
,5
,6
]}

机构：

[1] Hefei Univ Technol, Sch Mat Sci & Engn, Hefei 230009, Peoples R China

[2] Univ Cincinnati, Dept Chem & Environm Engn, Cincinnati, OH 45221 USA

[3] Hefei Comprehens Natl Sci Ctr, Inst Energy, Anhui Energy Lab, Hefei 230009, Peoples R China

[4] Hefei Univ Technol, Key Lab Adv Funct Mat & Devices Anhui Prov, Hefei 230009, Peoples R China

[5] Hefei Univ Technol, China Int S&T Cooperat Base Adv Energy & Environm, Hefei 230009, Peoples R China

[6] Hefei Univ Technol, Anhui Prov Int S&T Cooperat Base Adv Energy, Hefei 230009, Peoples R China

来源：

ISCIENCE | 2024年 / 27卷 / 06期

基金：

中国博士后科学基金; 中国国家自然科学基金;

关键词：

ELECTROCHEMICAL CO2 REDUCTION; PULSED ELECTROREDUCTION; MULTICARBON PRODUCTS; COPPER SURFACE; CU; ELECTRODES; CATALYSTS; OPERANDO; GAS; SPECTROSCOPY;

D O I：

10.1016/j.isci.2024.110005

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

Electrocatalysts undergo structural evolution under operating electrochemical CO2 reduction reaction (CO2RR) conditions. This dynamic reconstruction correlates with variations in CO2RR activity, selectivity, and stability, posing challenges in catalyst design for electrochemical CO2RR. Despite increased research on the reconstruction behavior of CO2RR electrocatalysts, a comprehensive understanding of their dynamic structural evolution under reaction conditions is lacking. This review summarizes recent developments in the dynamic reconstruction of catalysts during the CO2RR process, covering fundamental principles, modulation strategies, and in situ/operando characterizations. It aims to enhance understanding of electrocatalyst dynamic reconstruction, offering guidelines for the rational design of CO2RR electrocatalysts.

引用

页数：24

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