Spatial Distribution, Speciation, and Ecological Risk Assessment of Heavy Metals in Surface Sediments of Dongjiang Lake, Hunan Province

被引:0
|
作者
Zhang T.-L. [1 ,2 ]
Yi L.-X. [1 ]
Li C.-C. [3 ]
Yuan S.-S. [4 ]
Dou Y.-X. [5 ]
Tian S.-Y. [1 ]
Lin K.-X. [2 ]
机构
[1] Tianjin Marine Environmental Protection and Restoration Technology Engineering Center, Key Laboratory of Marine Resources Chemistry and Food Technology, Ministry of Education, College of Marine and Environmental Sciences, Tianjin University of Science and
[2] State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing
[3] Chenzhou Ecological and Environmental Monitoring Center, Chenzhou
[4] Chenzhou Dongjiang Lake Water Environment Protection Bureau, Chenzhou
[5] Chenzhou Municipal Ecology and Environment Bureau, Chenzhou
来源
Huanjing Kexue/Environmental Science | 2023年 / 44卷 / 09期
关键词
Dongjiang Lake; ecological risk; heavy metal; sediment; speciation;
D O I
10.13227/j.hjkx.202209060
中图分类号
学科分类号
摘要
To understand the heavy metal pollution status of Dongjiang Lake, the contents and species of heavy metals in the surface sediments were investigated during September 2021, and the heavy metal pollution level and potential ecological risk were evaluated. The results showed that Cd, Pb, As, Cu, Zn, Ni, and Cr contents were in the range of 0. 40-34. 1, 14. 8-1 688, 6. 99-1 155, 6. 89-280, 26. 2-1 739, 6. 29-55. 4, and 23. 3-44. 8 mg·kg - 1 , respectively, with extremely uneven spatial distributions. The highest contents of Cd, Pb, As, Zn, Cu, and Ni were found in the site adjacent to Yaogangxian tungsten ore. The proportion of metal species with bioavailability was high, in which Cd in acid-soluble species was 46. 7%-71. 5% and Pb in reducible species was 46. 8%-67. 0%. The bioavailable species of Cu, Zn, Ni, and Cr were 35%-68%, 42%-72%, 26%-51%, and 6%-30%, respectively, although they primarily existed in residual species. According to the geo-accumulation index (Igeo ), there was a moderate or extreme pollution status of Cd in all sites, moderate or extreme pollution status of Pb in 90% of sites, and moderate pollution status of As, Cu, and Zn in 30% of sites. The ecological risk factor (Eir ) of Cd showed high potential ecological risk in all sites with significantly high potential ecological risk in 80% of sites. Moreover, As and Pb had significantly high potential ecological risk, and Cu had moderate potential ecological risk in S7, which was adjacent to Yaogangxian tungsten ore. There was a high total potential ecological risk in all sites and significantly high potential ecological risk in 50% of sites. Therefore, the surface sediments of Dongjiang Lake were under the combined pollution of Cd, Pb, As, Zn, and Cu with high bioavailability and high total potential ecological risk. © 2023 Science Press. All rights reserved.
引用
收藏
页码:4898 / 4905
页数:7
相关论文
共 45 条
  • [21] Ma J H, Han C X, Jiang Y L., Some problems in the application of potential ecological risk index, Geographical Research, 39, 6, pp. 1233-1241, (2020)
  • [22] Fern佗ndez J A, Carballeira A., Evaluation of contamination, by different elements, in terrestrial mosses [J], Archives of Environmental Contamination and Toxicology, 40, 4, pp. 461-468, (2001)
  • [23] H覽kanson L., The quantitative impact of pH, bioproduction and Hg-contamination on the Hg-content of fish (pike), Environmental Pollution Series B, Chemical and Physical, 1, 4, pp. 285-304, (1980)
  • [24] Sun Z H, Xie X D, Wang P, Et al., Heavy metal pollution caused by small-scale metal ore mining activities: a case study from a polymetallic mine in South China, Science of the Total Environment, 639, pp. 217-227, (2018)
  • [25] Sheng W K, Hou Q Y, Yang Z F, Et al., Distribution characteristics and ecological risk assessment of heavy metals in sediments from Xiang River, China Environmental Science, 39, 5, pp. 2230-2240, (2019)
  • [26] Lu S J, Wang Y Y, He L H., Heavy metal pollution and ecological risk assessment of the paddy soils near a smelting area in Hunan Province, Environmental Monitoring in China, 31, 3, pp. 77-83, (2015)
  • [27] Tessier A, Campbell P G C, Bisson M., Sequential extraction procedure for the speciation of particulate trace metals, Analytical Chemistry, 51, 7, pp. 844-851, (1979)
  • [28] De Jonge M, Teuchies J, Meire P, Et al., The impact of increased oxygen conditions on metal-contaminated sediments part II: effects on metal accumulation and toxicity in aquatic invertebrates, Water Research, 46, 10, pp. 3387-3397, (2012)
  • [29] Campana O, Blasco J, Simpson S L., Demonstrating the appropriateness of developing sediment quality guidelines based on sediment geochemical properties, Environmental Science & Technology, 47, 13, pp. 7483-7489, (2013)
  • [30] Davidson C M, Thomas R P, McVey S E, Et al., Evaluation of a sequential extraction procedure for the speciation of heavy metals in sediments, Analytica Chimica Acta, 291, 3, pp. 277-286, (1994)