HYDROGEN-BOND COOPERATIVITY AND FREE-VOLUME EFFECTS ON NORMAL AND SUPERCOOLED WATER SELF-DIFFUSION

被引：9

作者：

LAMANNA, R ^{[1
]}

CANNISTRARO, S ^{[1
]}

机构：

[1] UNIV TUSCIA, DIPARTIMENTO SCI AMBIENTALI, SEZ CHIM & FIS, VITERBO, ITALY

来源：

PHYSICAL REVIEW A | 1992年 / 46卷 / 12期

关键词：

D O I：

10.1103/PhysRevA.46.R7367

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

The interpretation of the experimental self-diffusion data on normal and supercooled water has been revisited in the light of both the recently reported evidence for a temperature-dependent H-bond cooperativity and the free-volume fluctuations within the water percolative patches. The proposed model, which is consistent with the presence of a continuity of states between liquid and solid phases, was found to fit the NMR experimental data to an accuracy comparable to that obtained by a power law.

引用

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页码：R7367 / R7370

页数：4

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