MOLECULAR AXIS ORIENTATION AND TRANSITIONAL PATH EFFECTS IN THE ROTATIONAL STRUCTURE OF MULTIPHOTON TRANSITIONS

被引:0
|
作者
MAINOS, C
机构
[1] Laboratoire de Physique des Lasers, Université Paris-Nord, Villetaneuse, 93430, Av. J. B. Clément
关键词
D O I
10.1080/00268979100101901
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The intensity distribution among the rotational branches in a multiphoton process is considered. It is shown that the excitation probability of a rotational line depends drastically on the transitional path involved as well as on the molecular axis orientation. Each transitional path derives a distinct rotational structure and the intensity distribution of the rotational branches in the excitation spectra reveals the dominant transitional path.
引用
收藏
页码:1241 / 1255
页数:15
相关论文
共 45 条
  • [1] Multiorder rotational Raman transitions in molecular alignment and orientation
    Xu, Shuwu
    Lian, Zhenzhong
    Hong, Qian-Qian
    Wang, Lingxiao
    Chen, Huajie
    Huang, Yunxia
    Shu, Chuan-Cun
    PHYSICAL REVIEW A, 2024, 110 (02)
  • [2] INTERFERENCE EFFECTS IN THE ROTATIONAL ORIENTATION OF MOLECULAR PHOTOFRAGMENTS
    BESWICK, JA
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1992, 204 : 252 - PHYS
  • [3] Entanglement of molecular-orientation, rotational and orbital degrees of freedom in multiphoton orientational wave packets
    Mainos, C.
    Dutier, G.
    Grucker, J.
    Perales, F.
    Baudon, J.
    Ducloy, M.
    JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2008, 41 (03)
  • [4] DEGENERATE MULTIPHOTON PARAMETRIC SCATTERING OF THE IR RADIATION AT VIBRATION-ROTATIONAL MOLECULAR-TRANSITIONS
    BOLOTSKIKH, LT
    POPKOV, VG
    POPOV, AK
    SHALAEV, VM
    KVANTOVAYA ELEKTRONIKA, 1986, 13 (05): : 942 - 949
  • [5] SUPERNOVA SHOCK TRIGGERING AND INJECTION INTO THE PRESOLAR CLOUD: EFFECTS OF ROTATIONAL AXIS ORIENTATION
    Boss, A. P.
    Keiser, S. A.
    METEORITICS & PLANETARY SCIENCE, 2015, 50
  • [6] Controlling molecular orientation through radiative rotational transitions in strong static electric fields
    Mayle, Michael
    Gonzalez-Ferez, Rosario
    Schmelcher, Peter
    PHYSICAL REVIEW A, 2007, 75 (01):
  • [7] MOLECULAR BEAM INVESTIGATION OF ROTATIONAL TRANSITIONS .2. THE ROTATIONAL LEVELS OF KBR AND THEIR HYPERFINE STRUCTURE
    FABRICAND, BP
    CARLSON, RO
    LEE, CA
    RABI, II
    PHYSICAL REVIEW, 1953, 91 (06): : 1403 - 1408
  • [8] MOLECULAR BEAM INVESTIGATION OF ROTATIONAL TRANSITIONS .1. THE ROTATIONAL LEVELS OF KCL AND THEIR HYPERFINE STRUCTURE
    LEE, CA
    FABRICAND, BP
    CARLSON, RO
    RABI, II
    PHYSICAL REVIEW, 1953, 91 (06): : 1395 - 1403
  • [9] ROTATIONAL EFFECTS IN COLLISIONALLY INDUCED FINE-STRUCTURE TRANSITIONS
    BAYLIS, WE
    WALENTYNOWICZ, E
    PHANEUF, RA
    KRAUSE, L
    PHYSICAL REVIEW LETTERS, 1973, 31 (12) : 741 - 744
  • [10] THE SINGLE PATH ROTATIONAL STRUCTURE OF N-PHOTON TRANSITIONS IN DIATOMIC-MOLECULES
    MAINOS, C
    CASTEX, MC
    MOLECULAR PHYSICS, 1989, 68 (03) : 615 - 628