INFLUENCES OF CLOUD PHOTOCHEMICAL PROCESSES ON TROPOSPHERIC OZONE

被引:292
|
作者
LELIEVELD, J
CRUTZEN, PJ
机构
[1] Max Planck Institute for Chemistry, Division of Atmospheric Chemistry, D-6500 Mainz
关键词
D O I
10.1038/343227a0
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Global models of atmospheric chemistry typically neglect the chemical effects of clouds. Although clouds occupy only about 15% of the volume of the lower troposphere, and the volume fraction of liquid water in clouds is only 10-7 to 10-6, aqueous-phase chemistry is shown to decrease significantly ozone concentrations in the troposphere. Hydroxyl, formaldehyde and nitrogen oxide concentrations are decreased as well, thereby reducing the oxidation and cleansing efficiency of the troposphere and influencing the atmospheric budgets of many trace gases. © 1990 Nature Publishing Group.
引用
收藏
页码:227 / 233
页数:7
相关论文
共 50 条
  • [1] PHOTOCHEMICAL THEORY OF TROPOSPHERIC OZONE
    CHAMEIDES, W
    WALKER, JCG
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH, 1973, 78 (36): : 8751 - 8760
  • [2] PHOTOCHEMICAL THEORY OF TROPOSPHERIC OZONE
    CHAMEIDES, W
    WALKER, JCG
    [J]. TRANSACTIONS-AMERICAN GEOPHYSICAL UNION, 1973, 54 (11): : 1098 - 1098
  • [3] PHOTOCHEMICAL THEORY OF TROPOSPHERIC OZONE
    CHAMEIDE.W
    WALKER, JCG
    [J]. TRANSACTIONS-AMERICAN GEOPHYSICAL UNION, 1973, 54 (12): : 1293 - 1293
  • [4] LATITUDINAL VARIATION OF TROPOSPHERIC OZONE IN A PHOTOCHEMICAL MODEL
    HAMEED, S
    STEWART, RW
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS, 1983, 88 (NC9) : 5153 - 5162
  • [5] Influences of oceanic ozone deposition on tropospheric photochemistry
    Pound, Ryan J.
    Sherwen, Tomas
    Helmig, Detlev
    Carpenter, Lucy J.
    Evans, Mat J.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (07) : 4227 - 4239
  • [6] An Eulerian photochemical model for tropospheric ozone over the tropics
    Debaje, SB
    Jadhav, DB
    [J]. CURRENT SCIENCE, 1999, 77 (11): : 1537 - 1541
  • [7] LATITUDINAL VARIATION OF TROPOSPHERIC OZONE IN A PHOTOCHEMICAL MODEL.
    Hameed, Sultan
    Stewart, Richard W.
    [J]. Journal of Geophysical Research, 1983, 88 (C9): : 5153 - 5162
  • [8] Numerical Study of Cloud Effects on Tropospheric Ozone
    Bin Zhu
    Hui Xiao
    Meiyuan Huang
    Zihua Li
    [J]. Water, Air, and Soil Pollution, 2001, 129 : 199 - 216
  • [9] Numerical study of cloud effects on tropospheric ozone
    Zhu, B
    Xiao, H
    Huang, MY
    Li, ZH
    [J]. WATER AIR AND SOIL POLLUTION, 2001, 129 (1-4): : 199 - 216
  • [10] TROPOSPHERIC OZONE CHEMISTRY - THE IMPACT OF CLOUD CHEMISTRY
    JONSON, JE
    ISAKSEN, ISA
    [J]. JOURNAL OF ATMOSPHERIC CHEMISTRY, 1993, 16 (02) : 99 - 122