Optical-microphysical and physical-chemical characteristics of Siberian biomass burning: Experiments in Aerosol Chamber

被引：26

作者：

Popovicheva O.B. ^{[1
]}

Kozlov V.S. ^{[2
]}

Rakhimov R.F. ^{[2
]}

Shmargunov V.P. ^{[2
]}

Kireeva E.D. ^{[1
]}

Persiantseva N.M. ^{[1
]}

Timofeev M.A. ^{[1
]}

Engling G. ^{[3
]}

Eleftheriadis K. ^{[4
]}

Diapouli E. ^{[4
]}

Panchenko M.V. ^{[2
]}

Zimmermann R. ^{[5
,6
,7
]}

Schnelle-Kreis J. ^{[6
,7
]}

机构：

[1] Skobeltsyn Research Institute of Nuclear Physics, Moscow State University, Moscow

[2] V. E. Zuev Institute of Atmospheric Optics, Siberian Branch, Russian Academy of Sciences, Tomsk

[3] National Tsing Hua University, Hsinchu

[4] Institute of Nuclear and Radiological Science & Technology, Energy & Safety N.C.S.R. “Demokritos”, Environmental Radioactivity Laboratory, Attiki

[5] Joint Mass Spectrometry Center, Cooperation Group Comprehensive Molecular Analytics, Helmholtz Zentrum Muenchen, Neuherberg

[6] Joint Mass Spectrometry Center, Chair of Analytical Chemistry, Institute of Chemistry University of Rostock, Rostock

[7] Helmholtz Virtual Institute of Complex Molecular Systems in Environmental Health (HICE), Rostock

来源：

Atmospheric and Oceanic Optics | 2016年 / 29卷 / 6期

关键词：

Large Aerosol Chamber; mixed-phase burning; open flaming; Siberian biomasses; smoke particle characteristics; smokes; smoldering;

D O I：

10.1134/S1024856016060129

中图分类号：

学科分类号：

摘要：

A series of experiments aimed at studying the effect of combustion regimes of typical Siberian biomasses on the optical, microphysical, and physical-chemical properties of smoke aerosols was performed in the Large Aerosol Chambe, Institute of Atmospheric Optics, Siberian Branch, Russian Academy of Sciences. A comprehensive data analysis showed that temperature regime of Siberian pine and coniferous tree burning has a key effect on the formation and time dynamics of all smoke characteristics. The polarization spectronephelometer measurements of light scattering are used to determine the size distributions and absorption indices of particles. Particles in the smoldering phase are weakly absorbing, but the mixed phase contains a strongly absorbing fine component produced in open flame phases. We studied microstructure characteristics of aerosols by the analysis of morphology and elemental composition. Groups of soot and organic particles were determined as micromarkers of emissions in open flaming and smoldering phases, respectively. The organic and elemental carbon contents, origin and concentration of chemical compounds in the water-soluble ion fraction exhibit a strong dependence on the combustion phase. Sugar anhydride (levoglucosan) was determined in the smoldering phase as a stable molecular marker of Siberian pine burning. A number of specific markers of coniferous wood burning were identified among the chemical compounds. Smoke aging is accompanied by condensation of organic and inorganic compounds, transformation of aerosol surface chemistry, and the formation of the group of potassium-rich particles, all demonstrating the complexity and variability of the chemical composition and microstructure of atmospheric aerosol pollution during Siberian forest fires. © 2016, Pleiades Publishing, Ltd.

引用

页码：492 / 500

页数：8

共 40 条

[1] Dynamics of optical-microphysical characteristics of smokes from Siberian wildfires in the Big Aerosol Chamber at the stages of smoke generation and ageing
Kozlov, V. S.
Konovalov, I. B.
Uzhegov, V. N.
Chernov, D. G.
Pol'kin, Vas V.
Zenkova, P. N.
Yausheva, E. P.
Shmargunov, V. P.
Dubtsov, S. N.
[J]. 26TH INTERNATIONAL SYMPOSIUM ON ATMOSPHERIC AND OCEAN OPTICS, ATMOSPHERIC PHYSICS, 2020, 11560
[2] Chemical Composition and Toxicity of Siberian Biomass Burning in the Large Aerosol Chamber (Tomsk)
A. V. Semenova
Yu. A. Zavgorodnyaya
M. A. Chichaeva
V. S. Kozlov
O. B. Popovicheva
[J]. Atmospheric and Oceanic Optics, 2022, 35 : S38 - S47
[3] Chemical Composition and Toxicity of Siberian Biomass Burning in the Large Aerosol Chamber (Tomsk)
Semenova, A. V.
Zavgorodnyaya, Yu. A.
Chichaeva, M. A.
Kozlov, V. S.
Popovicheva, O. B.
[J]. ATMOSPHERIC AND OCEANIC OPTICS, 2022, 35 (SUPPL 1) : S38 - S47
[4] Smoke aerosol chemistry and aging of Siberian biomass burning emissions in a large aerosol chamber
Kalogridis, A. -C.
Popovicheva, O. B.
Engling, G.
Diapouli, E.
Kawamura, K.
Tachibana, E.
Ono, K.
Kozlov, V. S.
Eleftheriadis, K.
[J]. ATMOSPHERIC ENVIRONMENT, 2018, 185 : 15 - 28
[5] TEMPORAL dynamics of optical-microphysical characteristics of atmospheric aerosol at the Spitsbergen Archipelago in 2011-2014
Chernov, D. G.
Kozlov, V. S.
Panchenko, M. V.
Turchinovich, Yu. S.
Radionov, V. F.
Gubin, A. V.
Prakhov, A. N.
[J]. 21ST INTERNATIONAL SYMPOSIUM ON ATMOSPHERIC AND OCEAN OPTICS: ATMOSPHERIC PHYSICS, 2015, 9680
[6] Impact of combustion phase on scattering and spectral absorption of Siberian biomass burning: studies in Large Aerosol Chamber
Popovicheva, O. B.
Kozlov, V. S.
[J]. 26TH INTERNATIONAL SYMPOSIUM ON ATMOSPHERIC AND OCEAN OPTICS, ATMOSPHERIC PHYSICS, 2020, 11560
[7] Chemical and physical transformations of organic aerosol from the photo-oxidation of open biomass burning emissions in an environmental chamber
Hennigan, C. J.
Miracolo, M. A.
Engelhart, G. J.
May, A. A.
Presto, A. A.
Lee, T.
Sullivan, A. P.
McMeeking, G. R.
Coe, H.
Wold, C. E.
Hao, W. -M.
Gilman, J. B.
Kuster, W. C.
de Gouw, J.
Schichtel, B. A.
Collett, J. L., Jr.
Kreidenweis, S. M.
Robinson, A. L.
[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (15) : 7669 - 7686
[8] Aerosol Optical Characteristics During the Biomass Burning Season in Southeastern Mexico
Giovanni Carabalí
Blanca Ríos
Lizeth Florean-Cruz
Héctor Estévez
Mauro Valdés-Barrón
Roberto Bonifaz
David Riveros-Rosas
[J]. Water, Air, & Soil Pollution, 2019, 230
[9] Aerosol Optical Characteristics During the Biomass Burning Season in Southeastern Mexico
Carabali, Giovanni
Rios, Blanca
Florean-Cruz, Lizeth
Estevez, Hector
Valdes-Barron, Mauro
Bonifaz, Roberto
Riveros-Rosas, David
[J]. WATER AIR AND SOIL POLLUTION, 2019, 230 (10):
[10] Inferring the absorption properties of organic aerosol in Siberian biomass burning plumes from remote optical observations
Konovalov, Igor B.
Golovushkin, Nikolai A.
Beekmann, Matthias
Panchenko, Mikhail V.
Andreae, Meinrat O.
[J]. ATMOSPHERIC MEASUREMENT TECHNIQUES, 2021, 14 (10) : 6647 - 6673

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