Non-collinear magnetic configuration mediated exchange coupling at the interface of antiferromagnet and rare-earth nanolayers

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Junyu Huang
Chang Liu
Yifan Cui
Yuxiang Ling
Keming Chen
Kunlong Zhao
Xiangshang Xiao
Bin Yuan
Amitesh Paul
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[1] Guangdong Technion-Israel Institute of Technology,Department of Materials Science and Engineering, and Guangdong Provincial Key Laboratory of Materials and Technologies for Energy Conversion
[2] Technion-Israel Institute of Technology,Department of Materials Science and Engineering
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Scientific Reports | / 12卷
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Mn3\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$_{3}$$\end{document}Ir/CoFe bilayer is a prototypical exchange-coupled antiferromagnet (AF)–ferromagnet (FM) system. Nevertheless, a strong exchange coupling between FM and rare-earth(RE) interfaces of Fe/Dy and Fe/Tb has been established earlier. Strong coupling at the FM–RE interface originates from the number of irreversible spins owing to the imbalance in the non-collinear configuration in RE. However, exchange coupling between AF–RE could not be established due to the minimal number of irreversible spins in AF and RE. A frustrated inter-domain magnetic interaction leads to the coexistence of spin-freezing-like ordering around the temperature range of helical spin modulation at the exchange-coupled interfaces of RE-based specimens. To overcome the lack of coupling between the AF–RE interface, we use a sandwich structure of AF–FM–RE layers (Mn3\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$_{3}$$\end{document}Ir/CoFe/Dy) as we demonstrate establishing considerable exchange bias in the system. Changing the bias direction during field cooling introduces possible differences in non-collinear directions (helicities), which affects the number of irreversible spins and consequent exchange coupling differently for opposite directions. The non-collinear structures in RE are topologically stable; thus, their directions of orientation can be regarded as an additional degree of freedom, which can be manipulated in all-spin-based technology.
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