Visible-light-induced regioselective cross-dehydrogenative coupling of 2-isothiocyanatonaphthalenes with amines using molecular oxygen

被引:0
|
作者
Ziyu Gan
Guoqing Li
Xiaobo Yang
Qiuli Yan
Guiyun Xu
Gaoyang Li
Yuan-Ye Jiang
Daoshan Yang
机构
[1] Qingdao University of Science and Technology,Key Laboratory of Optic
[2] Qufu Normal University,electric Sensing and Analytical Chemistry for Life Science, Ministry of Education, Shandong Key Laboratory of Biochemical Analysis; College of Chemistry and Molecular Engineering
[3] Shenyang Normal University,School of Chemistry and Chemical Engineering
[4] Qingdao West Coast New Area Poli Junior Middle School,Institute of Catalysis for Energy and Environment, College of Chemistry & Chemical Engineering
来源
Science China Chemistry | 2020年 / 63卷
关键词
visible light; cross-dehydrogenative coupling; C-S bond; synthetic methods; metal-free;
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学科分类号
摘要
An efficient and eco-friendly protocol for the construction of naphtho[2,1-d]thiazol-2-amines through visible-light photoredoxcatalyzed C(sp2)-H/S-H cross-dehydrogenative coupling reactions between 2-isothiocyanatonaphthalenes and amines was established. In this reaction, the new C-N and C-S bonds are formed simultaneously in a single step. This new method provides a straightforward approach for constructing valuable sulfur-containing compounds. [graphic not available: see fulltext]
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页码:1652 / 1658
页数:6
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