Mode-coupling approximation in a fractional-power generalization: Particle dynamics in supercooled liquids and glasses

被引:0
|
作者
A. V. Mokshin
A. V. Chvanova
R. M. Khusnutdinoff
机构
[1] Kazan (Volga Region) Federal University,
来源
Theoretical and Mathematical Physics | 2012年 / 171卷
关键词
space-time correlation; vitrification; nonergodicity; mode-coupling approximation; disordered system; projection operator; integro-differential equation;
D O I
暂无
中图分类号
学科分类号
摘要
We describe the particle dynamics in supercooled liquids in the mode-coupling approximation in a fractional-power generalization, where the kinetic integro-differential equations are exactly derived from the equations of motion of the dynamical variables by projection operator methods. We show that in the case of separated time scales in the particle dynamics and with the nonlinear interaction between the stochastic and translation motion modes taken into account, the solution of the equations gives a well-defined picture of singularities of the one-particle dynamics of supercooled liquids and glasses. Comparison with the data for the metal alloy Fe50Cr50 atomic dynamics simulation demonstrates a good agreement in the entire temperature range corresponding to the supercooled liquid and glass phases.
引用
收藏
页码:541 / 552
页数:11
相关论文
共 50 条
  • [1] Mode-coupling approximation in a fractional-power generalization: Particle dynamics in supercooled liquids and glasses
    Mokshin, A. V.
    Chvanova, A. V.
    Khusnutdinoff, R. M.
    THEORETICAL AND MATHEMATICAL PHYSICS, 2012, 171 (01) : 541 - 552
  • [2] Non-equilibrium mode-coupling theory for supercooled liquids and glasses
    Latz, A
    JOURNAL OF PHYSICS-CONDENSED MATTER, 2000, 12 (29) : 6353 - 6363
  • [3] RELAXATIONAL DYNAMICS IN SUPERCOOLED LIQUIDS - EXPERIMENTAL TESTS OF THE MODE-COUPLING THEORY
    CUMMINS, HZ
    LI, G
    DU, WM
    HERNANDEZ, J
    PHYSICA A-STATISTICAL MECHANICS AND ITS APPLICATIONS, 1994, 204 (1-4) : 169 - 201
  • [4] Mode-coupling theory for the shear viscosity in supercooled liquids
    Franosch, T
    Gotze, W
    PHYSICAL REVIEW E, 1998, 57 (05) : 5833 - 5840
  • [5] Mode-coupling theory and the glass transition in supercooled liquids
    Das, SP
    REVIEWS OF MODERN PHYSICS, 2004, 76 (03) : 785 - 851
  • [6] Orientational dynamics in supercooled liquids near Tc and comparison with ideal mode-coupling theory
    Hinze, G
    Brace, DD
    Gottke, SD
    Fayer, MD
    PHYSICAL REVIEW LETTERS, 2000, 84 (11) : 2437 - 2440
  • [7] Supercooled liquids under shear: A mode-coupling theory appraoch
    Miyazaki, K
    Yamamoto, R
    Reichman, DR
    SLOW DYNAMICS IN COMPLEX SYSTEMS, 2004, 708 : 635 - 638
  • [8] Molecular mode-coupling theory for supercooled liquids: Application to water
    Fabbian, L
    Latz, A
    Schilling, R
    Sciortino, F
    Tartaglia, P
    Theis, C
    PHYSICAL REVIEW E, 1999, 60 (05): : 5768 - 5777
  • [9] Structural relaxation in quantum supercooled liquids: A mode-coupling approach
    Das, Ankita
    Rabani, Eran
    Miyazaki, Kunimasa
    Harbola, Upendra
    JOURNAL OF CHEMICAL PHYSICS, 2021, 154 (01):
  • [10] DYNAMICS OF SUPERCOOLED WATER - MODE-COUPLING THEORY APPROACH
    SOKOLOV, AP
    HURST, J
    QUITMANN, D
    PHYSICAL REVIEW B, 1995, 51 (18): : 12865 - 12868