The development of electronics is increasingly dependent on low-cost, flexible, solution-processed semiconductors. Colloidal quantum dots are solution-processed semiconducting nanocrystals that have a size-tunable bandgap and can be fabricated on a range of substrates. Here we review developments in colloidal quantum dot electronics, focusing on luminescent, optoelectronic, memory and thermoelectric devices. We examine the role of surface chemistry in the suppression of non-radiative processes, the control of light–matter interactions and the regulation of carrier transport properties. We also highlight the prospects of perovskite quantum dots as single-photon sources, the design of new classes of colloidal quantum dots and superlattices for emerging applications and the role of hybrid device architectures in compensating for the limited carrier mobility in colloidal quantum dot solids while maintaining their tunable spectral response.
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Tsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China
MIT, Dept Chem, Cambridge, MA 02139 USA
CALTECH, Dept Phys, Pasadena, CA 91125 USATsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China
Bao, Jie
Bawendi, Moungi G.
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MIT, Dept Chem, Cambridge, MA 02139 USATsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China
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Los Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA
Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87131 USALos Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA
Park, Young-Shin
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Roh, Jeongkyun
Diroll, Benjamin T.
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Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL USALos Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA
Diroll, Benjamin T.
Schaller, Richard D.
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Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL USA
Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL USALos Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA
Schaller, Richard D.
Klimov, Victor I.
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Los Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USALos Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA
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King Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi ArabiaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Masala, Silvia
Adinolfi, Valerio
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Univ Toronto, Dept Elect & Comp Engn, Toronto, ON M5S 3G4, CanadaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Adinolfi, Valerio
Sun, Jon-Paul
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Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 4R2, CanadaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Sun, Jon-Paul
Del Gobbo, Silvano
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King Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi ArabiaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Del Gobbo, Silvano
Voznyy, Oleksandr
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Univ Toronto, Dept Elect & Comp Engn, Toronto, ON M5S 3G4, CanadaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Voznyy, Oleksandr
Kramer, Illan J.
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Univ Toronto, Dept Elect & Comp Engn, Toronto, ON M5S 3G4, CanadaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Kramer, Illan J.
Hill, Ian G.
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Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 4R2, CanadaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
Hill, Ian G.
Sargent, Edward H.
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Univ Toronto, Dept Elect & Comp Engn, Toronto, ON M5S 3G4, CanadaKing Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia