The development and evaluation of microstructured reactors for the water gas shift and preferential oxidation reactions in the 5 kW range

被引：29
|
作者：
O'Connell, Martin [1 ]
Kolb, Gunther [1 ]
Schelhaas, Karl-Peter [1 ]
Schuerer, Jochen [1 ]
Tiemann, David [1 ]
Ziogas, Athanassios [1 ]
Hessel, Volker [1 ,2 ]
机构：
[1] Inst Mikrotech Mainz GmbH, D-55129 Mainz, Germany
[2] Eindhoven Univ Technol TU E, Dept Chem & Chem Engn, NL-5600 MB Eindhoven, Netherlands
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2010年 / 35卷 / 06期
关键词：
Water gas shift; Preferential oxidation; Microchannels; CO clean-up; FUEL-CELL APPLICATIONS; CO SELECTIVE OXIDATION; MICROCHANNEL REACTOR; HYDROGEN-PRODUCTION; CATALYSTS; DEACTIVATION; MICROREACTOR; PERFORMANCE; PROCESSOR; MECHANISM;
D O I：
10.1016/j.ijhydene.2009.12.113
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
5 kW(el) One-Stage Water Gas Shift (WGS) and Preferential Oxidation (PROx) reactors were designed and evaluated for the clean-up of surrogate diesel reformate. For the WGS reactor, CO conversions of up to 95% were attained using typical surrogate synthetic diesel reformate. The PROx reactor was capable of converting a feed concentration of 1.0 mol% CO to 20 ppm. Load changes for both reactors could be carried out without significant overshoots of carbon monoxide. (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：2317 / 2327
页数：11
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