Undesired Reactions in Aqueous Rechargeable Zinc Ion Batteries

被引：213

作者：

Verma, Vivek ^{[1
]}

Kumar, Sonal ^{[1
]}

Manalastas, William, Jr. ^{[1
]}

Srinivasan, Madhavi ^{[1
,2
]}

机构：

[1] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

[2] Nanyang Technol Univ, Energy Res Inst NTU ERI N, Singapore 637553, Singapore

来源：

ACS ENERGY LETTERS | 2021年 / 6卷 / 05期

基金：

新加坡国家研究基金会;

关键词：

SURFACE-CHARGE DENSITY; ELECTROCHEMICAL PERFORMANCE; DENDRITE FORMATION; CRYSTAL-STRUCTURE; CATHODE MATERIAL; ELECTROLYTE; METAL; STORAGE; MECHANISM; EVOLUTION;

D O I：

10.1021/acsenergylett.1c00393

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Rechargeable zinc-ion batteries (RZIBs) utilizing aqueous electrolytes can offer high safety, low cost, and fast charge/discharge ratings for large-scale energy storage. The use of water as electrolyte solvent facilitates low cost, facile processing, reduced safety concerns, and fast ion kinetics. However, free water molecules also instigate many simultaneously occurring undesired reactions in the RZIB system, leading to capacity fade and limited operational lifetime. Here, our review traces each undesired reaction and its cascade of detrimental ramifications on RZIB cycling. We discuss balancing merits, reported strategies, and future perspectives to mitigate these undesired reactions and further improve the RZIBs' operational lifetimes.

引用

页码：1773 / 1785

页数：13

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