Aqueous leaching of Cr2O3-doped UO2 spent nuclear fuel under oxidizing conditions

被引：4
|
作者：
Barreiro-Fidalgo, Alexandre [1 ]
Roth, Olivia [1 ]
Evins, Lena Zetterstrom [2 ]
Spahiu, Kastriot [2 ]
机构：
[1] Studsvik Nucl AB, S-61182 Nykoping, Sweden
[2] Swedish Nucl Fuel & Waste Management Co SKB, S-16903 Solna, Sweden
来源：
MRS ADVANCES | 2021年 / 6卷 / 4-5期
关键词：
The Swedish nuclear Fuel and Waste Management Company (SKB) is greatly acknowledged for financial support. The authors would like to thank Framatome for their contribution in this project. Special thanks to everyone involved in this project at Studsvik for their excellent work;
D O I：
10.1557/s43580-021-00043-y
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
Understanding the leaching behavior of spent nuclear fuel is crucial for the safety assessment of deep geological repositories to dispose spent nuclear fuel. During the last decades, new types of nuclear fuel are being introduced in commercial reactors. These new fuels with additives such as chromium oxide (Cr2O3) have an impact on the UO2 microstructure and therefore might affect properties relevant to the safety assessment. The main goal of this investigation is to understand the effects of Cr-doping on the instant release fraction of fission products. A sample consisting of fuel fragments and separated cladding was leached in simplified groundwater under aerated conditions at Studsvik's Hot Cell Laboratory. Data from leaching experiments performed on Cr-doped fuel manufactured by Framatome are presented and compared to other commercial Cr-doped fuel manufactured by Westinghouse (Advanced DOped Pellet Technology, ADOPT) and standard UO2 fuel.
引用
收藏
页码：103 / 106
页数：4
相关论文
共 50 条
  • [1] Aqueous leaching of Cr2O3-doped UO2 spent nuclear fuel under oxidizing conditions
    Alexandre Barreiro-Fidalgo
    Olivia Roth
    Lena Zetterström Evins
    Kastriot Spahiu
    MRS Advances, 2021, 6 : 103 - 106
  • [2] Spent fuel UO2 matrix alteration in aqueous media under oxidizing conditions
    Jegou, C.
    Muzeau, B.
    Broudic, V.
    Roudil, D.
    Deschanels, X.
    RADIOCHIMICA ACTA, 2007, 95 (09) : 513 - 522
  • [3] Aqueous leaching of ADOPT and standard UO2 spent nuclear fuel under H2 atmosphere
    Fidalgo, Alexandre Barreiro
    Roth, Olivia
    Puranen, Anders
    Evins, Lena Z.
    Spahiu, Kastriot
    MRS ADVANCES, 2020, 5 (3-4) : 167 - 175
  • [4] Aqueous leaching of ADOPT and standard UO2 spent nuclear fuel under H2 atmosphere
    Alexandre Barreiro Fidalgo
    Olivia Roth
    Anders Puranen
    Lena Z. Evins
    Kastriot Spahiu
    MRS Advances, 2020, 5 : 167 - 175
  • [5] Aqueous leaching of ADOPT and standard UO2 spent nuclear fuel under H2 atmosphere
    Fidalgo A.B.
    Roth O.
    Puranen A.
    Evins L.Z.
    Spahiu K.
    1600, Springer Nature (05): : 167 - 175
  • [6] Behavior of UO2 in the RBMK-1000 spent fuel under oxidizing conditions
    Kolyadin, AB
    Mishin, VY
    Mishin, KY
    Aloy, AS
    Koltsova, TI
    SCIENTIFIC BASIS FOR NUCLEAR WASTE MANAGEMENT XXVIII, 2004, 824 : 119 - 125
  • [7] Aqueous leaching of high burnup UO2 fuel under hydrogen conditions
    Puranen, Anders
    Roth, Olivia
    Evins, Lena Z.
    Spahiu, Kastriot
    MRS ADVANCES, 2018, 3 (19): : 1013 - 1018
  • [8] Aqueous leaching of high burnup UO2 fuel under hydrogen conditions
    Anders Puranen
    Olivia Roth
    Lena Z. Evins
    Kastriot Spahiu
    MRS Advances, 2018, 3 (19) : 1013 - 1018
  • [9] Factors governing microstructure development of Cr2O3-doped UO2 during sintering
    Bourgeois, L
    Dehaudt, P
    Lemaignan, C
    Hammou, A
    JOURNAL OF NUCLEAR MATERIALS, 2001, 297 (03) : 313 - 326
  • [10] Dynamic leaching studies of 48 MWd/kgU UO2 commercial spent nuclear fuel under oxic conditions
    Serrano-Purroy, D.
    Casas, I.
    Gonzalez-Robles, E.
    Glatz, J. P.
    Wegen, D. H.
    Clarens, F.
    Gimenez, J.
    de Pablo, J.
    Martinez-Esparza, A.
    JOURNAL OF NUCLEAR MATERIALS, 2013, 434 (1-3) : 451 - 460
12345