Excited-state absorption dynamics in polymethine dyes detected by polarization-resolved pump-probe measurements

被引:41
|
作者
Lepkowicz, RS [1 ]
Przhonska, OV
Hales, JM
Hagan, DJ
Van Stryland, EW
Bondar, MV
Slominsky, YL
Kachkovski, AD
机构
[1] Univ Cent Florida, CREOL, Sch Opt, Orlando, FL 32816 USA
[2] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev 28, Ukraine
[3] Natl Acad Sci Ukraine, Inst Organ Chem, UA-02094 Kiev 94, Ukraine
关键词
excited-state absorption; polymethine dye; rotational motion; orientation of transition dipole moments; anisotropy;
D O I
10.1016/S0301-0104(02)00937-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Polarization-resolved excitation-probe measurements are performed for a new series of polymethine dyes in several solvents and a polyurethane acrylate elastopolymer. We describe our experimental studies and give an analysis of the nature of the rotational motions of excited molecules and orientation of the excited-state transitions relative to transitions from the ground state. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:277 / 291
页数:15
相关论文
共 50 条
  • [1] Polarization-resolved pump-probe spectroscopy with high harmonics
    Mairesse, Y.
    Haessler, S.
    Fabre, B.
    Higuet, J.
    Boutu, W.
    Breger, P.
    Constant, E.
    Descamps, D.
    Mevel, E.
    Petit, S.
    Salieres, P.
    NEW JOURNAL OF PHYSICS, 2008, 10
  • [2] A time resolved double pump-probe experimental technique to characterize excited-state parameters of organic dyes
    Swatton, SNR
    Welford, KR
    Hollins, RC
    Sambles, JR
    APPLIED PHYSICS LETTERS, 1997, 71 (01) : 10 - 12
  • [3] Polarization-Resolved Pump-Probe Spectroscopy with High Order Harmonics
    Mevel, E.
    Mairesse, Y.
    Haessler, S.
    Fabre, B.
    Higuet, J.
    Bouti, W.
    Breger, P.
    Constant, E.
    Descamps, D.
    Petit, S.
    Shafir, D.
    Delcon, H.
    Dudovich, N.
    Salieres, P.
    ULTRAFAST PHENOMENA XVI, 2009, 92 : 24 - +
  • [4] Determining Excited-State Absorption Properties of a Quinoid Flavin by Polarization-Resolved Transient Spectroscopy
    Xu, Yi
    Peschel, Martin T.
    Jaenchen, Miriam
    Foja, Richard
    Storch, Golo
    Thyrhaug, Erling
    de Vivie-Riedle, Regina
    Hauer, Juergen
    JOURNAL OF PHYSICAL CHEMISTRY A, 2024, 128 (19): : 3830 - 3839
  • [5] Polarization-resolved femtosecond pump-probe spectroscopy for Au nanodisks at the LSP resonance
    Sugita, Atsushi
    Yogo, Hirofumi
    Mochizuki, Kannta
    Hamada, Shohei
    Matsui, Hiroumi
    Ono, Atsushi
    Inami, Wataru
    Kawata, Yoshimasa
    Yoshizawa, Masayuki
    OSA CONTINUUM, 2020, 3 (10) : 2943 - 2952
  • [6] Approximate calculation of femtosecond pump-probe spectra monitoring nonadiabatic excited-state dynamics
    Dilthey, S
    Hahn, S
    Stock, G
    JOURNAL OF CHEMICAL PHYSICS, 2000, 112 (11): : 4910 - 4922
  • [7] Quantitative Decoupling of Excited-State Absorption Cross Section and Population via Pump-Probe Spectroscopy with a Strong Probe
    Barker, Alex J.
    Hodgkiss, Justin M.
    PHYSICAL REVIEW APPLIED, 2015, 4 (02):
  • [8] Shining Light on the Solution- and Excited-State Dynamics of Chalcogenopyrylium Polymethine Dyes
    Rosch, Lauren E.
    Crawley, Matthew R.
    O'Donnell, Ryan M.
    Rohrabaugh, Thomas N., Jr.
    Ensley, Trenton R.
    Sobiech, Thomas A.
    Cook, Timothy R.
    ORGANOMETALLICS, 2022, 41 (16) : 2301 - 2316
  • [9] On the calculation of rotational anisotropy decay, as measured by ultrafast polarization-resolved vibrational pump-probe experiments
    Lin, Y. -S.
    Pieniazek, P. A.
    Yang, Mino
    Skinner, J. L.
    JOURNAL OF CHEMICAL PHYSICS, 2010, 132 (17):
  • [10] Ultrafast pump-probe studies of excited-state charge-transfer dynamics in blue copper proteins
    Book, LD
    Arnett, DC
    Hu, HB
    Scherer, NF
    JOURNAL OF PHYSICAL CHEMISTRY A, 1998, 102 (23): : 4350 - 4359