Local spin moment configuration in the frustrated s=1/2 Heisenberg triangular antiferromagnet V15 determined by NMR

被引:32
|
作者
Furukawa, Yuji [1 ]
Nishisaka, Yusuke
Kumagai, Ken-ich
Kogerler, Paul
Borsa, Ferdinando
机构
[1] Hokkaido Univ, Grad Sch Sci, Div Phys, Sapporo, Hokkaido 0600810, Japan
[2] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA
[3] Iowa State Univ, Ames Lab, Ames, IA 50011 USA
[4] INFM, Dipartimento Fis A Volta, I-127100 Pavia, Italy
[5] INFM, Unita CNISM, I-127100 Pavia, Italy
基金
美国国家卫生研究院;
关键词
D O I
10.1103/PhysRevB.75.220402
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report very low-temperature measurements of V-51 NMR spectra as a function of external magnetic field in the s=1/2 Heisenberg triangular antiferromagnet cluster K-6[V15As6O42(H2O)]center dot 8H(2)O (V15), a simple prototype of a geometrically magnetic frustrated system. It is known that the frustration is relieved by a splitting of the degenerate ground state into two S-T=1/2 states. Our measurements allow the microscopic determination of the local spin configuration both in the nonfrustrated total spin S-T=3/2 state at high fields and in the two quasidegenerate S-T=1/2 ground states at low fields, where it is shown that the simple frustrated chiral configuration in the triangle is broken down into two different spin configurations corresponding to the two quasidegenerate S-T=1/2 states.
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页数:4
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