Sorption of lead ion by layered double hydroxide intercalated with diethylenetriaminepentaacetic acid

被引：110
|
作者：
Liang, Xuefeng [1 ,2 ,3 ]
Hou, Wanguo [4 ]
Xu, Yingming [1 ,2 ,3 ]
Sun, Guohong [5 ]
Wang, Lin [1 ,2 ,3 ]
Sun, Yang [1 ,2 ,3 ]
Qin, Xu [1 ,2 ,3 ]
机构：
[1] Minist Agr, Dept Pollut Control, Agroenvironm Protect Inst, Tianjin 300191, Peoples R China
[2] Minist Agr, Key Lab Prod Environm & Agroprod Safety, Tianjin 300191, Peoples R China
[3] Tianjin Key Lab Agroenvironm & Food Safety, Tianjin 300191, Peoples R China
[4] Shandong Univ, Key Lab Colloid & Interface Chem, Educ Minist, Jinan 250100, Peoples R China
[5] Tianjin Agr Univ, Dept Elementary Sci, Tianjin 300384, Peoples R China
来源：
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS | 2010年 / 366卷 / 1-3期
基金：
国家高技术研究发展计划(863计划); 中国国家自然科学基金;
关键词：
Layered double hydroxide; Diethylenetriaminepentaacetic acid; Lead; Sorption; CHELATING-AGENTS; AQUEOUS-SOLUTION; ANIONIC CLAYS; METAL-IONS; ADSORPTION; REMOVAL; PB(II); SURFACE; CU2+; PB2+;
D O I：
10.1016/j.colsurfa.2010.05.012
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Mg2Al layered double hydroxide (Mg2Al LDH) samples intercalated with diethylenetriaminepentaacetic acid (DTPA) (Mg2Al-DTPA LDH in short) were prepared by co-precipitation and well characterized by XRD, SEM, TEM, IR and XPS. The sorption behaviors and mechanisms of Pb2+ on the samples were studied in detail while Mg2Al-Cl LDH as a reference. The maximum sorption amounts were about 170 and 40 mg/g for Mg2Al-DTPA LDH and Mg2Al-Cl LDH, respectively. Langmuir isotherm was proved to describe the sorption data better and pseudo-second order kinetic model could fit the sorption kinetic processes better for both LDHs samples. The mechanisms of Pb2+ sorption on Mg2Al-DTPA LDH can be explained by Pb-DTPA chelating while that for Mg2Al-Cl LDH is primary surface-induced precipitation. The Mg2Al-DTPA LDH could provide a potential remedy for heavy metal contamination in soils and water. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码：50 / 57
页数：8
相关论文
共 50 条
  • [1] Efficient adsorption of Mn(Ⅱ) by layered double hydroxides intercalated with diethylenetriaminepentaacetic acid and the mechanistic study
    Mingjie Huang
    Yingxin Zhang
    Wei Xiang
    Tao Zhou
    Xiaohui Wu
    Juan Mao
    [J]. Journal of Environmental Sciences, 2019, (11) : 56 - 65
  • [2] Removal of lead from aqueous solution on glutamate intercalated layered double hydroxide
    Shen Yanming
    Liu Dongbin
    Li Shifeng
    Fan Lihui
    Chen Shuai
    Haque, Md Atiqul
    [J]. ARABIAN JOURNAL OF CHEMISTRY, 2017, 10 : S2295 - S2301
  • [3] Preparation of layered double hydroxide intercalated by Gallic acid for boron adsorption
    Cai, Liang
    Zhang, Yuze
    Peng, Xiaowu
    Guo, Fan
    Ji, Lianmin
    Li, Lijuan
    [J]. JOURNAL OF WATER PROCESS ENGINEERING, 2021, 44
  • [4] The preparation and characterization of sulfamic acid-intercalated layered double hydroxide
    Jiang, Yu
    Gu, Xiaoyu
    Zhang, Sheng
    Tang, Wufei
    Zhao, Jingran
    [J]. MATERIALS LETTERS, 2015, 150 : 31 - 34
  • [5] Selective adsorption of mercury ion by mercaptocarboxylic acid intercalated Mg-Al layered double hydroxide
    Nakayama, H.
    Hirami, S.
    Tsuhako, M.
    [J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2007, 315 (01) : 177 - 183
  • [6] Efficient adsorption of Mn(II) by layered double hydroxides intercalated with diethylenetriaminepentaacetic acid and the mechanistic study
    Huang, Mingjie
    Zhang, Yingxin
    Xiang, Wei
    Zhou, Tao
    Wu, Xiaohui
    Mao, Juan
    [J]. JOURNAL OF ENVIRONMENTAL SCIENCES, 2019, 85 : 56 - 65
  • [7] Sorption-desorption processes in the system of U(VI)-layered double hydroxide intercalated with EDTA
    Goncharuk, V. V.
    Pshinko, G. N.
    Puzyrnaya, L. N.
    [J]. JOURNAL OF WATER CHEMISTRY AND TECHNOLOGY, 2012, 34 (02) : 88 - 95
  • [8] Sorption-desorption processes in the system of U(VI)-layered double hydroxide intercalated with EDTA
    V. V. Goncharuk
    G. N. Pshinko
    L. N. Puzyrnaya
    [J]. Journal of Water Chemistry and Technology, 2012, 34 : 88 - 95
  • [9] Intercalative Ion-Exchange Route to Amino Acid Layered Double Hydroxide Nanohybrids and Their Sorption Properties
    Choi, Goeun
    Yang, Jae-Hun
    Park, Ga-Young
    Vinu, Ajayan
    Elzatahry, Ahmad
    Yo, Chul Hyun
    Choy, Jin-Ho
    [J]. EUROPEAN JOURNAL OF INORGANIC CHEMISTRY, 2015, (06) : 925 - 930
  • [10] Enhanced sorption of perfluorooctanoic acid with organically functionalized layered double hydroxide
    Min, Xiaopeng
    Huo, Jingwan
    Dong, Qianqian
    Xu, Shangping
    Wang, Yin
    [J]. CHEMICAL ENGINEERING JOURNAL, 2022, 446
12345