The electro-Fenton regeneration of Granular Activated Carbons: Degradation of organic contaminants and the relationship to the carbon surface

被引:55
|
作者
Bury, Naomi A. [1 ]
Mumford, Kathryn A. [1 ]
Stevens, Geoffrey W. [1 ]
机构
[1] Univ Melbourne, Dept Chem Engn, Parkville, Vic 3010, Australia
关键词
Electro-Fenton; Granular Activated Carbon; Regeneration; Surface chemistry; Porosity; SOLAR PHOTOELECTRO-FENTON; ADVANCED OXIDATION PROCESSES; MALACHITE GREEN-DYE; ACID AQUEOUS-MEDIUM; ELECTROCHEMICAL REGENERATION; HYDROGEN-PEROXIDE; IRON-OXIDE; EFFICIENT MINERALIZATION; PARTICLE ELECTRODES; AROMATIC-COMPOUNDS;
D O I
10.1016/j.jhazmat.2021.125792
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Electrochemical regeneration of Granular Activated Carbon is an emerging treatment option to restore adsorption capacity in systems designed to remove organic contaminants from aqueous solutions. The electro-Fenton process is one such electrochemical process and it is reviewed along with other members of its family including Photoelectro-Fenton and Heterogeneous electro-Fenton and electro-Fenton like reactions, for its ability to regenerate Granular Activated Carbons contaminated with organics. The behaviour of critical operating parameter such as pH, current, catalyst concentration and initial contaminant concentration are reviewed to find optimal operating conditions. The relationship between electro-Fenton regeneration and the chemical and physical surface of the carbon is also explored. Understanding regeneration mechanisms and the optimal operating conditions enables these technologies to be used commercially and to be scaled-up and treat contaminated waters more efficiently.
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页数:18
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