Sequential simulation of dense oxygen permeation membrane reactor for hydrogen production from oxidative steam reforming of ethanol with ASPEN PLUS

被引：27

作者：

Jin, Yun ^{[1
]}

Rui, Zebao ^{[1
]}

Tian, Ye ^{[1
]}

Lin, Yuesheng ^{[2
]}

Li, Yongdan ^{[1
]}

机构：

[1] Tianjin Univ, Sch Chem Engn, Tianjin Key Lab Catalysis Sci & Technol, Tianjin 300072, Peoples R China

[2] Arizona State Univ, Dept Chem Engn, Tempe, AZ 85287 USA

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2010年 / 35卷 / 13期

关键词：

Dense tubular membrane reactor; Sequential simulation; Oxidative steam reforming of ethanol; Oxygen permeation; NOBLE-METAL CATALYSTS; METHANE CONVERSION; PERMEABLE MEMBRANE; CHEMICAL-REACTIONS; CERAMIC MEMBRANES; OXIDE MEMBRANES; BA0.5SR0.5CO0.8FE0.2O3-DELTA; BED; PERFORMANCE; STABILITY;

D O I：

10.1016/j.ijhydene.2010.04.042

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Hydrogen production via oxidative steam reforming of ethanol in a dense tubular membrane reactor (DMR) is sequentially simulated with ASPEN PLUS. The DMR is divided into multi-sub-reactors, and the Gibbs free energy minimization sub-model in ASPEN PLUS is employed to simulate the oxidative steam reforming of ethanol process in the subreactors. A FORTRAN sub-routine is integrated into ASPEN PLUS to simulate the oxygen permeation through membranes in the sub-separators. The simulation result indicates that there is an optimal length of the tubular membrane reactor at the operating temperature and steam-to-ethanol (H2O/EtOH) ratio, under which hydrogen and carbon monoxide formation reach their maxima. (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.

引用

页码：6691 / 6698

页数：8

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