Chitosan assisted MXene decoration onto polymer fabric for high efficiency solar driven interfacial evaporation of oil contaminated seawater

被引:40
|
作者
Wu, Zefeng [1 ]
Li, Juntao [1 ]
Zhang, Shu [1 ]
Yan, Jun [1 ]
Gao, Jiefeng [1 ,2 ,3 ]
Zheng, Nan [4 ]
Xue, Huaiguo [1 ]
机构
[1] Yangzhou Univ, Sch Chem & Chem Engn, 180 Rd Siwangting, Yangzhou 225002, Jiangsu, Peoples R China
[2] Sichuan Univ, State Key Lab Polymer Mat Engn, 24,South Sect 1,First Ring Rd, Chengdu 610065, Sichuan, Peoples R China
[3] Hangzhou Normal Univ, Key Lab Organosilicon Chem & Mat Technol, Minist Educ, Bldg 22,2318 Yuhangtang Rd,Cangqian St, Hangzhou 311121, Peoples R China
[4] Dalian Polytech Univ, Sch Light Ind & Chem Engn, Dalian 116034, Peoples R China
关键词
Solar driven interfacial evaporation; Fabric; MXene; Chitosan; Crude oil; DESALINATION; TECHNOLOGY; OXIDATION; FUTURE; ENERGY;
D O I
10.1016/j.jcis.2022.04.074
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The solar-driven interfacial evaporation (SDIE) is now a promising way to solve the shortage of fresh water. However, high performance SDIE for the oil contaminated seawater remains challenging. Here, we propose a facile ``chitosan assisted MXene decoration" strategy to prepare a superhydrophilic and underwater superoleophobic Chitosan/MXene/fabric (CMF) for highly efficient SDIE. Benefiting from the superhydrophilicity and excellent photo-thermal conversion performance, the CMF is served as both the solar absorber and the water transportation path. Under the light illumination with one sun intensity (1 kW.m(-2)), a high evaporation rate of 1.50 kg.m(-2)h(-1) and efficiency of 88.05% are achieved. The strong interfacial interaction and outstanding salt rejection behavior of the CMF ensure the SDIE long-term stability and durability. In addition, the underwater superoleophobic CMF can effectively and quickly repel different oils and is hence suitable for high performance SDIE of the oil-in-water emulsion and the crude oil contaminated seawater. This work provides a rational design and optimization for the SDIE system, which holds great potential in practical desalination applications. (C) 2022 Elsevier Inc. All rights reserved.
引用
收藏
页码:169 / 180
页数:12
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