Enhanced Visible Light Driven Photocatalytic Behavior of BiFeO3/Reduced Graphene Oxide Composites

被引:60
|
作者
Si, Yun-hui [1 ,2 ]
Xia, Yu [1 ,2 ]
Shang, Shao-ke [1 ,2 ]
Xiong, Xin-bo [1 ,2 ]
Zeng, Xie-rong [1 ,2 ]
Zhou, Ji [3 ]
Li, Ya-yun [1 ,2 ]
机构
[1] Shenzhen Univ, Coll Mat Sci & Engn, Shenzhen Key Lab Special Funct Mat, Shenzhen 518060, Peoples R China
[2] Shenzhen Univ, Coll Mat Sci & Engn, Shenzhen Engn Lab Adv Technol Ceram, Shenzhen 518060, Peoples R China
[3] Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
基金
中国国家自然科学基金;
关键词
BiFeO3; reduced graphene oxide; photocatalytic; visible light; AQUEOUS-SOLUTION; DEGRADATION; FERROMAGNETISM; MICROSPHERES; FABRICATION; NANORODS; ACID;
D O I
10.3390/nano8070526
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
BiFeO3/Reduced Graphene Oxide (BFO/RGO) composites have been fabricated by a simple hydrothermal method. The X-ray diffraction (XRD), scanning electron microscopy (SEM), Raman, and X-ray photoelectron spectroscopy (XPS) analysis reveal that graphene oxide was reduced in hydrothermal process and BFO/RGO composites were successfully synthesized. UV-visible absorption and photoluminescence properties show that the introduction of RGO can effectively reduce the recombination of photogenerated electron and hole pairs. Compared to the pristine BFO, the photocatalytic performance of BiFeO3 Graphene Oxide (BGO) composites is enhanced for the degradation of Methylene blue (MB) solution under visible light irradiation, and the result shows that the optimal amount of Graphene Oxide (GO) in the composites is 60 mg (BG060). The excellent photocatalytic performance is mainly ascribed to improved light absorption, increased reactive sites, and the low recombination rate of electron-hole pairs. This work can provide more insights into designing advanced photocatalysts for wastewater treatment and environmental protection.
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页数:12
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