Mobile laboratory with rapid response instruments for real-time measurements of urban and regional trace gas and particulate distributions and emission source characteristics
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作者:
Kolb, CE
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Kolb, CE
Herndon, SC
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Herndon, SC
McManus, B
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
McManus, B
Shorter, JH
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Shorter, JH
Zahniser, MS
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Zahniser, MS
Nelson, DD
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Nelson, DD
Jayne, JT
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Jayne, JT
Canagaratna, MR
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Canagaratna, MR
Worsnop, DR
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机构:Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
Worsnop, DR
机构:
[1] Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA
[2] Aerodyne Res Inc, Ctr Aerosol & Cloud Chem, Billerica, MA 01821 USA
Recent technological advances have allowed the development of robust, relatively compact, low power, rapid response (similar to1 s) instruments with sufficient sensitivity and specificity to quantify many trace gases and aerosol particle components in the ambient atmosphere. Suites of such instruments can be deployed on mobile platforms to study atmospheric processes, map concentration distributions of atmospheric pollutants, and determine the composition and intensities of emission sources. A mobile laboratory containing innovative tunable infrared laser differential absorption spectroscopy (TILDAS) instruments to measure selected trace gas concentrations at sub parts-per-billion levels and an aerosol mass spectrometer (AMS) to measure size resolved distributions of the nonrefractory chemical components of fine airborne particles as well as selected commercial fast response instruments and position/velocity sensors is described. Examples of the range of measurement strategies that can be undertaken using this mobile laboratory are discussed, and samples of measurement data are presented.