All-Optical Control of the Ultrafast Dynamics of a Hybrid Plasmonic System

被引：63
|
作者：
Utikal, Tobias [1 ,2 ,3 ]
Stockman, Mark I. [1 ,2 ,3 ,4 ]
Heberle, Albert P. [1 ,2 ]
Lippitz, Markus [1 ,2 ,3 ]
Giessen, Harald [1 ,2 ]
机构：
[1] Univ Stuttgart, Inst Phys 4, D-70550 Stuttgart, Germany
[2] Univ Stuttgart, Res Ctr SCoPE, D-70550 Stuttgart, Germany
[3] Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany
[4] Georgia State Univ, Dept Phys & Astron, Atlanta, GA 30303 USA
来源：
PHYSICAL REVIEW LETTERS | 2010年 / 104卷 / 11期
关键词：
COHERENT CONTROL; TIME; ENHANCEMENT; FIELDS; DECAY; GAAS;
D O I：
10.1103/PhysRevLett.104.113903
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We demonstrate complete all-optical and phase-stable control of the linear optical polarization and the nonlinear coherent response (third-harmonic generation) of a hybrid nanoplasmonic-photonic system. A few tens of femtoseconds after the excitation, we turn the response on and off at any given point in time and probe its temporal evolution throughout the control process with a three-pulse nonlinear optical technique. After being switched off, the polarization and the nonlinear radiation remain off permanently. All experiments agree well with numerical simulations based on a damped harmonic oscillator model.
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页数：4
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