Anisotropic Evaporator with a T-Shape Design for High-Performance Solar-Driven Zero-Liquid Discharge

被引:49
|
作者
Liu, Hanwen [1 ]
Jin, Ruizhi [2 ]
Duan, Sicong [1 ]
Ju, Yujun [1 ]
Wang, Zhuoyue [1 ]
Yang, Ke [1 ]
Wang, Baodui [1 ,2 ]
Wang, Bo [1 ,2 ]
Yao, Yonggang [3 ]
Chen, Fengjuan [1 ]
机构
[1] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou, Gansu, Peoples R China
[2] Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Western Chinas Environm Syst, Lanzhou 730000, Gansu, Peoples R China
[3] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc Die & Mold Technol, Wuhan 430074, Peoples R China
基金
中国国家自然科学基金;
关键词
solar desalination; T‐ shape design; water treatment; zero liquid discharge; EFFICIENT; WOOD; DESALINATION; GENERATION; MEMBRANE;
D O I
10.1002/smll.202100969
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Solar-driven evaporation is regarded as a sustainable wastewater treatment strategy for clean water recovery and salt condensation. However, achieving both high evaporation rate and long-term stability remain challenging due to poor thermal management and rapid salt accumulation and blocking. Here, a T-shape solar-driven evaporator, composed of a surface-carbonized longitudinal wood membrane (C-L-wood) is demonstrated as the top "-" for solar harvesting/vapor generation/salt collection and another piece of natural L-wood as the support for brine transporting and thermally insulating. The horizontally aligned micro-channels of C-L-wood have a low perpendicular thermal conductivity and can effectively localize the thermal energy for rapid evaporation. Meanwhile, the brine is guided to transport from the support L-wood to the centerline of the top evaporator and then toward the double edge ("-"), during which clean water is evaporated and salt is crystallized at the edge. The T-shape evaporator demonstrates a high evaporation rate of 2.43 kg m(-2) h(-1) under 1 sun irradiation, and is stable for 7 days of the outdoor operation, which simultaneously realizes clean water evaporation and salt collection (including Cu2+, CrO42-, Co2+), and achieves zero-liquid discharge. Therefore, the T-shape design provides an effective strategy for high performance wastewater treatment.
引用
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页数:9
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