Progress towards lead-free, efficient, and stable perovskite solar cells

被引:18
|
作者
Thornton, Sean T. [1 ]
Abdelmageed, Ghada [1 ]
Kahwagi, Rashad F. [1 ]
Koleilat, Ghada, I [1 ,2 ]
机构
[1] Dalhousie Univ, Dept Proc Engn & Appl Sci, 1360 Barrington St, Halifax, NS B3H 4R2, Canada
[2] Dalhousie Univ, Dept Elect & Comp Engn, 1360 Barrington St, Halifax, NS B3H 4R2, Canada
基金
加拿大创新基金会; 加拿大自然科学与工程研究理事会;
关键词
perovskite; solar cell; lead-free; stable; efficient; LIFE-CYCLE ASSESSMENT; TIN-BASED PEROVSKITE; ENHANCED PHOTOVOLTAIC PERFORMANCE; LIGHT-ABSORBING MATERIALS; FREE HALIDE PEROVSKITE; OPEN-CIRCUIT VOLTAGE; IODIDE PEROVSKITE; THIN-FILMS; IMPROVED STABILITY; BISMUTH IODIDE;
D O I
10.1002/jctb.6830
中图分类号
Q81 [生物工程学(生物技术)]; Q93 [微生物学];
学科分类号
071005 ; 0836 ; 090102 ; 100705 ;
摘要
Solar energy production requires an environmentally friendly, efficient, and stable light absorber. Perovskite solar cells (PSCs) have emerged as excellent candidate materials for photovoltaic (PV) energy conversion because of their low cost, ease of fabrication, flexibility, and versatility. However, typical high-efficiency PSCs, like methylammonium lead iodide (MAPbI(3)), rely on the use of the chemical lead (Pb), whose toxicity and detrimental impact on human health and the environment raise strong concerns. Therefore, less toxic substitutes that produce the same high performance as MAPbI(3) are of interest to enable a wide deployment of PSCs. Hence, much effort has focused on replacing Pb with other elements, such as tin (Sn), bismuth (Bi), antimony (Sb), and germanium (Ge) in perovskite materials, with the dual objectives of maintaining the superior optoelectronic properties of the perovskite and reducing its toxicity. In this review, the structure, optoelectronic properties, as well as recent advances in device performance of Pb-free PSCs are highlighted. Moreover, the stability challenges of Pb-free perovskite are detailed, and strategies to overcome them are discussed. Finally, a conclusion and outlook towards Pb-free perovskite photovoltaics (PV) is provided. (c) 2021 Society of Chemical Industry (SCI).
引用
收藏
页码:810 / 829
页数:20
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