Do you believe that atoms stay in place when you observe them in HREM?

被引:25
|
作者
Van Dyck, Dirk [1 ]
Lobato, Ivan [1 ]
Chen, Fu-Rong [2 ]
Kisielowski, Christian [3 ,4 ]
机构
[1] Univ Antwerp, EMAT, Groenenborgerlaan 171, B-2020 Antwerp, Belgium
[2] Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 300, Taiwan
[3] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA
[4] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA
关键词
Quantitative HREM; TDS; Dose rate dependence; ELECTRON-MICROSCOPE IMAGES; THERMAL DIFFUSE-SCATTERING; HIGH-RESOLUTION IMAGES; PHONON-SCATTERING; INELASTIC-SCATTERING; CONTRAST; DIFFRACTION; SIMULATIONS; SENSITIVITY; HOLOGRAPHY;
D O I
10.1016/j.micron.2014.09.003
中图分类号
TH742 [显微镜];
学科分类号
摘要
Recent advancements in aberration-corrected electron microscopy allow for an evaluation of unexpectedly large atom displacements beyond a resolution limit of similar to 0.5 angstrom, which are found to be dose-rate dependent in high resolution images. In this paper we outline a consistent description of the electron scattering process, which explains these unexpected phenomena. Our approach links thermal diffuse scattering to electron beam-induced object excitation and relaxation processes, which strongly contribute to the image formation process. The effect can provide an explanation for the well-known contrast mismatch ("Stobbs factor") between image calculations and experiments. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:158 / 163
页数:6
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