Self-organization of TiO2 microparticles on the surface of a thin liquid layer due to local heating and the formation of convective cells

被引:2
|
作者
Egorov, R., I [1 ]
Misyura, S. Y. [2 ]
Morozov, V. S. [2 ]
Zaitsev, A. S. [1 ]
机构
[1] Natl Res Tomsk Polytech Univ, 30 Lenin Ave, Tomsk 634050, Russia
[2] Russian Acad Sci, Siberian Branch, Kutateladze Inst Thermophys, 1 Lavrentyev Ave, Novosibirsk 630090, Russia
关键词
Benard-Marangoni convection; Self-assembly; Microparticles; Liquid interface; Laser heating;
D O I
10.1016/j.molliq.2020.114685
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The aggregation of TiO2 microparticles followed by self-organization of a cluster of agglomerates at convective cells formation in a thin layer of water is studied experimentally. Complex behavior of the cluster is considered at a strong system deviation from equilibrium as a result of local heating. A periodic character of the behavior of a cluster of particles has been detected. Particle sizes and the number of cells change cyclically over time. Hexagonal convective cells have a very small size of about 50-100 mu m(5-10 times less than the layer height). Data on the cluster occurrence and dissociation over time is provided. It is shown that when the particle diameter and the diameter of coagulated particles reach the maximum (the maximum diameter of the cluster corresponds to 100-130 mu m, and the maximum diameter of the aggregate is 20-30 mu m), the convective cells lose stability and the cluster partially disintegrates. Self-organization control using local heating can be effectively applied to create new materials, as well as in biology and medicine. (C) 2020 Elsevier B.V. All rights reserved.
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页数:10
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