Resonance lineshapes in two-dimensional Fourier transform spectroscopy

被引：121
|
作者：
Siemens, Mark E. [1 ,2 ]
Moody, Galan [1 ,2 ,3 ]
Li, Hebin [1 ,2 ]
Bristow, Alan D. [1 ,2 ]
Cundiff, Steven T. [1 ,2 ,3 ]
机构：
[1] Univ Colorado, JILA, Boulder, CO 80309 USA
[2] NIST, Boulder, CO 80309 USA
[3] Univ Colorado, Dept Phys, Boulder, CO 80309 USA
来源：
OPTICS EXPRESS | 2010年 / 18卷 / 17期
基金：
美国国家科学基金会;
关键词：
Fourier transforms;
D O I：
10.1364/OE.18.017699
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
We derive an analytical form for resonance lineshapes in two-dimensional (2D) Fourier transform spectroscopy. Our starting point is the solution of the optical Bloch equations for a two-level system in the 2D time domain. Application of the projection-slice theorem of 2D Fourier transforms reveals the form of diagonal and cross-diagonal slices in the 2D frequency data for arbitrary inhomogeneity. The results are applied in quantitative measurements of homogeneous and inhomogeneous broadening of multiple resonances in experimental data. (C) 2010 Optical Society of America
引用
收藏
页码：17699 / 17708
页数：10
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