Laser-induced interference, focusing, and diffraction of rescattering molecular photoelectrons

被引:102
|
作者
Yurchenko, SN [1 ]
Patchkovskii, S
Litvinyuk, IV
Corkum, PB
Yudin, GL
机构
[1] Natl Res Council Canada, Ottawa, ON K1A 0R6, Canada
[2] Kansas State Univ, JR Macdonald Lab, Manhattan, KS 66506 USA
[3] Univ Sherbrooke, Chim Theor Lab, Sherbrooke, PQ J1K 2R1, Canada
关键词
D O I
10.1103/PhysRevLett.93.223003
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We solve the time-dependent Schrodinger equation in three dimensions for H-2(+) in a one-cycle laser pulse of moderate intensity. We consider fixed nuclear positions and Coulomb electron-nuclear interaction potentials. We analyze the field-induced electron interference and diffraction patterns. To extract the ionization dynamics we subtract the excitations to low-lying bound states explicitly. We follow the time evolution of a well-defined wave packet that is formed near the first peak of the laser field. We observe the fragmentation of the wave packet due to molecular focusing. We show how to retrieve a diffraction molecular image by taking the ratio of the momentum distributions in the two lateral directions. The positions of the diffraction peaks are well described by the classical double slit diffraction rule.
引用
收藏
页码:223003 / 1
页数:4
相关论文
共 50 条
  • [1] Self-imaging of molecules from diffraction spectra by laser-induced rescattering electrons
    Xu, Junliang
    Chen, Zhangjin
    Le, Anh-Thu
    Lin, C. D.
    [J]. PHYSICAL REVIEW A, 2010, 82 (03):
  • [2] EVIDENCE FOR REVERSE PHOTOELECTRONS IN LASER-INDUCED CURRENT
    AHMAD, SR
    [J]. JOURNAL OF APPLIED PHYSICS, 1972, 43 (01) : 244 - &
  • [3] Large-angle electron diffraction structure in laser-induced rescattering from rare gases
    Ray, D.
    Ulrich, B.
    Bocharova, I.
    Maharjan, C.
    Ranitovic, P.
    Gramkow, B.
    Magrakvelidze, M.
    De, S.
    Litvinyuk, I. V.
    Le, A. T.
    Morishita, T.
    Lin, C. D.
    Paulus, G. G.
    Cocke, C. L.
    [J]. PHYSICAL REVIEW LETTERS, 2008, 100 (14)
  • [4] Ultrafast molecular imaging by laser-induced electron diffraction
    Peters, M.
    Nguyen-Dang, T. T.
    Cornaggia, C.
    Saugout, S.
    Charron, E.
    Keller, A.
    Atabek, O.
    [J]. PHYSICAL REVIEW A, 2011, 83 (05):
  • [5] Laser-induced electron diffraction: A tool for molecular orbital imaging
    Peters, M.
    Nguyen-Dang, T. T.
    Charron, E.
    Keller, A.
    Atabek, O.
    [J]. PHYSICAL REVIEW A, 2012, 85 (05):
  • [6] Imaging ultrafast molecular dynamics with laser-induced electron diffraction
    Blaga, Cosmin I.
    Xu, Junliang
    DiChiara, Anthony D.
    Sistrunk, Emily
    Zhang, Kaikai
    Agostini, Pierre
    Miller, Terry A.
    DiMauro, Louis F.
    Lin, C. D.
    [J]. NATURE, 2012, 483 (7388) : 194 - 197
  • [7] Imaging ultrafast molecular dynamics with laser-induced electron diffraction
    Cosmin I. Blaga
    Junliang Xu
    Anthony D. DiChiara
    Emily Sistrunk
    Kaikai Zhang
    Pierre Agostini
    Terry A. Miller
    Louis F. DiMauro
    C. D. Lin
    [J]. Nature, 2012, 483 : 194 - 197
  • [8] EFFECTS OF VARIATION OF THE LASER-PULSE WIDTH ON THE LASER-INDUCED PHOTOELECTRONS
    PARSA, Z
    [J]. NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1992, 318 (1-3): : 265 - 269
  • [9] Quantum effect of laser-induced rescattering from the tunneling barrier
    Han, Meng
    Ge, Peipei
    Fang, Yiqi
    Deng, Yongkai
    Wu, Chengyin
    Gong, Qihuang
    Liu, Yunquan
    [J]. PHYSICAL REVIEW A, 2019, 99 (02)
  • [10] Low-energy electron rescattering in laser-induced ionization
    Becker, W.
    Goreslavski, S. P.
    Milosevic, D. B.
    Paulus, G. G.
    [J]. JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2014, 47 (20)