Source apportionment of heavy metals in farmland soil of Wuwei, China: Comparison of three receptor models

被引:138
|
作者
Guan, Qingyu [1 ]
Zhao, Rui
Pan, Ninghui
Wang, Feifei
Yang, Yanyan
Luo, Haiping
机构
[1] Lanzhou Univ, Minist Educ, Key Lab Western Chinas Environm Syst, Lanzhou 730000, Gansu, Peoples R China
基金
中国国家自然科学基金;
关键词
Farmland soil heavy metals; Source apportionment; GPCA/APCS; PMF; UNMIX; HEALTH-RISK ASSESSMENT; POLYCYCLIC AROMATIC-HYDROCARBONS; PRINCIPAL COMPONENT SCORES; SOURCE IDENTIFICATION; AGRICULTURAL SOILS; TRACE-ELEMENTS; PARTICULATE MATTER; CONTAMINATED SOILS; POLLUTION CHARACTERISTICS; PHOSPHATE FERTILIZERS;
D O I
10.1016/j.jclepro.2019.117792
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Receptor models are, rarely utilized in soil but are often used to identify pollutant sources and quantify their contribution. This paper focuses on the soil in oasis farmland. A geochemical baseline is used to assess the pollution of the soil, and then three models are tentatively utilized to apportion heavy metals and compare the sources, the contributions and the operation effects. Pollution assessment indicated that the farmland soil of Wuwei was lightly contaminated by heavy metals. Source apportionments suggested that atmospheric deposition contributed the most pollution (53.95%-65.35%). The three models supplemented each other, and the grouped principal component analysis/absolute principal component scores (GPCA/APCS) was outstanding. GPCA/APCS and UNMIX suggested that agricultural activities were the prime anthropogenic source (51.06%-61.56%), followed by the combustion of fossil fuels (coal and oil) (27.92%-28.66%) and building materials-related activities source (10.52%-20.29%). Fertilizers and pesticides (67.88%-74.81%) contributed more than traffic emissions (25.19%-32.12%) in agricultural activities. Similar results were acquired via positive matrix factorization (PMF), while industrial activity was the highest individual contributor (29.91%). Therefore, combining these three models was the most effective approach, and more attention should be paid to mitigating the pollution caused by the use of fertilizers and pesticides as well as the industrial activities in Wuwei. The results of this study could provide reference in reduction of heavy metal pollution in farmland soil. (C) 2019 Elsevier Ltd. All rights reserved.
引用
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页数:10
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