Octadecanuclear Macrocycles and Nonanuclear Bowl-Shaped Structures Based on Two Analogous Pyridyl-Substituted Imidazole-4,5-dicarboxylate Ligands

被引：30

作者：

Zhang, Ying-Ying ^{[1
]}

Shen, Xu-Yu ^{[1
]}

Weng, Lin-Hong ^{[1
]}

Jin, Guo-Xin ^{[1
]}

机构：

[1] Fudan Univ, Dept Chem, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2014年 / 136卷 / 44期

基金：

美国国家科学基金会;

关键词：

METAL-ORGANIC FRAMEWORKS; CRYSTAL-STRUCTURES; COMPLEXES; COORDINATION; ZMOFS; HYDROGENATION; TETRANUCLEAR; ARCHITECTURE; ACTIVATION; POLYGONS;

D O I：

10.1021/ja5096914

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Two types of unprecedented Cp*Rh-based (Cp* = eta(5)-C5Me5) complexes, two octadecanuclear macrocycles, and a nonanuclear bowl-shaped complex have been synthesized from two analogous pyridyl-functionalized imidazole-4,5-dicarboxylate ligands, 2-(pyridin-4-yl)-1H-imidazole-4,5-dicarboxylate ligand and 2-(pyridin-3-yl)-1H-imidazole-4,5-dicarboxylate ligand, respectively.

引用

页码：15521 / 15524

页数：4

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