Probing a Critical Length Scale at the Glass Transition

被引:66
|
作者
Mosayebi, Majid [1 ]
Del Gado, Emanuela [1 ]
Ilg, Patrick [1 ]
Oettinger, Hans Christian [1 ]
机构
[1] ETH, Dept Mat, CH-8093 Zurich, Switzerland
关键词
FORMING LIQUIDS; SUPERCOOLED LIQUIDS; HETEROGENEOUS DYNAMICS; GROWING LENGTH; MIXTURE; ENTROPY;
D O I
10.1103/PhysRevLett.104.205704
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We give evidence of a clear structural signature of the glass transition, in terms of a static correlation length with the same dependence on the system size, which is typical of critical phenomena. Our approach is to introduce an external, static perturbation to extract the structural information from the system's response. In particular, we consider the transformation behavior of the local minima of the underlying potential energy landscape (inherent structures), under a static deformation. The finite-size scaling analysis of our numerical results indicate that the correlation length diverges at a temperature T(c), below the temperatures where the system can be equilibrated. Our numerical results are consistent with random first order theory, which predicts such a divergence with a critical exponent nu = 2/3 at the Kauzmann temperature, where the extrapolated configurational entropy vanishes.
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页数:4
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