High-Rate and High-Voltage Aqueous Rechargeable Zinc Ammonium Hybrid Battery from Selective Cation Intercalation Cathode

被引：68
|
作者：
Li, Chunyang [1 ,2 ]
Wu, Jianghua [3 ,4 ]
Ma, Fuxiang [1 ,2 ]
Chen, Yuhui [1 ,2 ]
Fu, Lijun [1 ,2 ]
Zhu, Yusong [1 ,2 ]
Zhang, Yi [1 ,2 ]
Wang, Peng [3 ,4 ]
Wu, Yuping [1 ,2 ]
Huang, Wei [1 ,2 ]
机构：
[1] Nanjing Tech Univ, Inst Adv Mat IAM, State Key Lab Mat Oriented Chem Engn, Nanjing 211816, Jiangsu, Peoples R China
[2] Nanjing Tech Univ, Coll Energy Sci & Engn, Nanjing 211816, Jiangsu, Peoples R China
[3] Nanjing Univ, Coll Engn & Appl Sci, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China
[4] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
来源：
ACS APPLIED ENERGY MATERIALS | 2019年 / 2卷 / 10期
关键词：
hybrid battery; Prussian blue analogue; ammonium-ion insertion; selective ion channel; high voltage; PRUSSIAN BLUE ANALOG; HIGH-ENERGY DENSITY; LIFE; ELECTROLYTE; HEXACYANOFERRATE; INSERTION; ANODE; NH4+;
D O I：
10.1021/acsaem.9b01469
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The shortage of lithium resources is promoting the development of cost-efficient battery candidates, especially aqueous rechargeable batteries (ARBs) with high safety and power density. Copper hexacyanoferrate (CuHCF) nanoparticles with high redox potential and rate capability is employed as the battery cathode for hosting ammonium-ion coupling with low-cost zinc anode. Benefiting from the selective ammoniumion channel in CuHCF, an aqueous rechargeable zinc ammonium hybrid battery is successfully engineered. It presents high . cell voltage (1.8 V), outstanding rate performance, low self-discharge, and satisfactory energy density of 114 Wh kg(-1) in consideration of total electrodes' active mass.
引用
收藏
页码：6984 / 6989
页数：11
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