Propagating Hybrid Tamm Exciton Polaritons in Organic Microcavity

被引:22
|
作者
Liu, Bin [1 ]
Wu, Rong [1 ,2 ]
Menon, Vinod M. [1 ,2 ]
机构
[1] CUNY City Coll, Dept Phys, New York, NY 10031 USA
[2] CUNY, Grad Ctr, Dept Phys, New York, NY 10016 USA
来源
JOURNAL OF PHYSICAL CHEMISTRY C | 2019年 / 123卷 / 43期
关键词
ENERGY-TRANSFER; SEMICONDUCTOR; GENERATION;
D O I
10.1021/acs.jpcc.9b06383
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Strong coupling between Tamm plasmons and organic cavity polaritons is observed at room temperature. Angle-resolved reflectometry experiments unambiguously indicate the anticrossing in the dispersion relations, which is characteristic of the strong coupling regime, and the Tamm plasmon-cavity polariton hybrid states can be energetically manipulated by tuning the Tamm plasmons. The experimental data are in good agreement with calculations based on the transfer matrix method. Emission from the lower energy Tamm plasmon cavity polariton hybrid states is observed, and the propagation property of the hybrid Tamm plasmon polariton is also studied. The real-space imaging experiments reveal that the propagation distance is larger when the Tamm plasmon and cavity polariton are strongly coupled in comparison to both the exciton of the uncoupled organic neat film and the cavity polaritons. Moreover, the propagation length of the hybrid polaritons increases as the fraction of Tamm plasmon component in the hybrid states increases.
引用
收藏
页码:26509 / 26515
页数:7
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