Full Lignin-Derived Electrospun Carbon Materials as Electrodes for Supercapacitors

被引:11
|
作者
Thielke, Michael W. [1 ]
Lopez Guzman, Stiven [2 ]
Victoria Tafoya, Jorge Pavel [1 ]
Garcia Tamayo, Esteban [2 ]
Castro Herazo, Cristina Isabel [2 ]
Hosseinaei, Omid [3 ]
Sobrido, Ana Jorge [1 ]
机构
[1] Queen Mary Univ London, Sch Engn & Mat Sci, London, England
[2] Univ Pontificia Bolivariana, Escuela Ingn, Medellin, Colombia
[3] RISE, Res Inst Sweden, Stockholm, Sweden
关键词
Lignin; Electropinning; supercapacitor; Biomass; sustainability; needleless electrospinning; in situ Raman; plasma-modified carbon; ACTIVATED CARBON; FUNCTIONAL-GROUPS; KRAFT LIGNIN; IRON-OXIDE; NANOFIBERS; PERFORMANCE; BIOMASS; FIBERS; XPS; STORAGE;
D O I
10.3389/fmats.2022.859872
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In the search for more sustainable energy storage devices, biomass-derived materials have been widely researched as carbon source for electrode applications. Here we present the processing of high molecular lignin, an abundant carbon rich biopolymer and byproduct of the pulp and paper industry, into freestanding nonwoven carbon fiber (CNFs) electrodes by using electrospinning. It is worth mentioning that no petrol-derived polymers that are usually included in the electrospinning of lignin, were employed in this work, making these electrodes more sustainable than common lignin-derived carbon electrodes. The effect of the carbonization temperature and oxygen plasma treatment in the electrochemical performance of the CNFs as electrodes for supercapacitors was studied. The upscaling of the processing of lignin into carbon electrodes was also explored by comparing a standard electrospinning set up with a needleless electrospinning equipment that enabled faster and higher throughput. The electrochemical performance of the CNFs increased after plasma treatment of the surface and the electrodes prepared using the standard set up exhibited the highest activity, achieving specific capacitances of up to 103.6 F g(-1).
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页数:10
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