Global mercury emissions to the atmosphere from anthropogenic and natural sources

被引:1061
|
作者
Pirrone, N. [1 ]
Cinnirella, S. [1 ]
Feng, X. [2 ]
Finkelman, R. B. [3 ]
Friedli, H. R. [4 ]
Leaner, J. [5 ]
Mason, R. [6 ]
Mukherjee, A. B. [7 ]
Stracher, G. B. [8 ]
Streets, D. G. [9 ]
Telmer, K. [10 ]
机构
[1] CNR, Inst Atmospher Pollut Res, Div Rende, Arcavacata Di Rende, Italy
[2] Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang, Peoples R China
[3] Univ Texas Dallas, Dallas, TX 75230 USA
[4] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[5] CSIR, Stellenbosch, South Africa
[6] Univ Connecticut, Dept Marine Sci, Hartford, CT 06112 USA
[7] Univ Helsinki, Dept Biol & Environm Sci, Helsinki, Finland
[8] E Georgia Coll, Div Sci & Math, Swainsboro, Georgia
[9] Argonne Natl Lab, Argonne, IL 60439 USA
[10] Univ Victoria, Sch Earth & Ocean Sci, Victoria, BC, Canada
关键词
FIRED POWER-PLANTS; MEDITERRANEAN REGION; VOLCANIC EMISSIONS; COAL COMBUSTION; FOREST-FIRES; UNCERTAINTIES; ACCUMULATION; CONSUMPTION; DEPOSITION; INVENTORY;
D O I
10.5194/acp-10-5951-2010
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This paper provides an up-to-date assessment of global mercury emissions from anthropogenic and natural sources. On an annual basis, natural sources account for 5207 Mg of mercury released to the global atmosphere, including the contribution from re-emission processes, which are emissions of previously deposited mercury originating from anthropogenic and natural sources, and primary emissions from natural reservoirs. Anthropogenic sources, which include a large number of industrial point sources, are estimated to account for 2320 Mg of mercury emitted annually. The major contributions are from fossil-fuel fired power plants (810 Mg yr(-1)), artisanal small scale gold mining (400 Mg yr(-1)), non-ferrous metals manufacturing (310 Mg yr(-1)), cement production (236 Mg yr(-1)), waste disposal (187 Mg yr(-1)) and caustic soda production (163 Mg yr(-1)). Therefore, our current estimate of global mercury emissions suggests that the overall contribution from natural sources (primary emissions + re-emissions) and anthropogenic sources is nearly 7527 Mg per year, the uncertainty associated with these estimates are related to the typology of emission sources and source regions.
引用
收藏
页码:5951 / 5964
页数:14
相关论文
共 50 条
  • [1] Mercury emissions to the atmosphere from natural and anthropogenic sources in the Mediterranean region
    Pirrone, N
    Costa, P
    Pacyna, JM
    Ferrara, R
    [J]. ATMOSPHERIC ENVIRONMENT, 2001, 35 (17) : 2997 - 3006
  • [2] Scenarios of global mercury emissions from anthropogenic sources
    Rafaj, P.
    Bertok, I.
    Cofala, J.
    Schoepp, W.
    [J]. ATMOSPHERIC ENVIRONMENT, 2013, 79 : 472 - 479
  • [3] Atmospheric mercury emissions in Australia from anthropogenic, natural and recycled sources
    Nelson, Peter F.
    Morrison, Anthony L.
    Malfroy, Hugh J.
    Cope, Martin
    Lee, Sunhee
    Hibberd, Mark L.
    Meyer, C. P.
    McGregor, John
    [J]. ATMOSPHERIC ENVIRONMENT, 2012, 62 : 291 - 302
  • [4] Annual emissions of mercury to the atmosphere from natural sources in Nevada and California
    Coolbaugh, MF
    Gustin, MS
    Rytuba, JJ
    [J]. ENVIRONMENTAL GEOLOGY, 2002, 42 (04): : 338 - 349
  • [5] Global emission of mercury to the atmosphere from anthropogenic sources in 2005 and projections to 2020
    Pacyna, E. G.
    Pacyna, J. M.
    Sundseth, K.
    Munthe, J.
    Kindbom, K.
    Wilson, S.
    Steenhuisen, F.
    Maxson, P.
    [J]. ATMOSPHERIC ENVIRONMENT, 2010, 44 (20) : 2487 - 2499
  • [6] Mercury emissions to the atmosphere from anthropogenic sources in Europe in 2000 and their scenarios until 2020
    Pacyna, Elisabeth G.
    Pacyna, Jozef M.
    Fudala, Janina
    Strzelecka-Jastrzab, Ewa
    Hlawiczka, Stanislaw
    Panasiuk, Damian
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2006, 370 (01) : 147 - 156
  • [7] GLOBAL INVENTORY OF NATURAL AND ANTHROPOGENIC EMISSIONS OF TRACE-METALS TO THE ATMOSPHERE
    NRIAGU, JO
    [J]. NATURE, 1979, 279 (5712) : 409 - 411
  • [8] COMPARISON OF THE FLUXES OF LEAD INTO THE ATMOSPHERE BY VOLCANOS AND ORGANIC EMISSIONS FROM TREES WITH OTHER NATURAL SOURCES AND WITH ANTHROPOGENIC SOURCES
    PATTERSON, CC
    [J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1979, (APR): : 137 - 137
  • [9] Global scenarios of anthropogenic mercury emissions
    Brocza, Flora Maria
    Rafaj, Peter
    Sander, Robert
    Wagner, Fabian
    Jones, Jenny Marie
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2024, 24 (12) : 7385 - 7404
  • [10] Composite global emissions of reactive chlorine from anthropogenic and natural sources: Reactive Chlorine Emissions Inventory
    Keene, WC
    Khalil, MAK
    Erickson, DJ
    McCulloch, A
    Graedel, TE
    Lobert, JM
    Aucott, ML
    Gong, SL
    Harper, DB
    Kleiman, G
    Midgley, P
    Moore, RM
    Seuzaret, C
    Sturges, WT
    Benkovitz, CM
    Koropalov, V
    Barrie, LA
    Li, YF
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D7) : 8429 - 8440