Charge order in quasi-one-dimensional organic charge-transfer solids

被引:1
|
作者
Clay, RT [1 ]
Campbell, DK
Mazumdar, S
机构
[1] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA
[2] Japan Sci & Technol Corp JST, ERATO Cooperat Excitat Project, Tucson, AZ 85721 USA
[3] Boston Univ, Dept Elect & Comp Engn, Boston, MA 02215 USA
[4] Boston Univ, Dept Phys, Boston, MA 02215 USA
关键词
organic conductors based on radical cation and/or anion salts; organic superconductors;
D O I
10.1016/S0379-6779(02)00782-8
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We examine two proposed models of the observed charge ordering (CO) in the quasi-1D, 1/4-filled organic charge transfer solids. The models are characterized by the site charge densities ..1010.. and ..1100.. respectively. Using a Peierls-extended Hubbard model to include both electron-electron and electron-phonon interactions, we show that 1) the ..1010.. CO can occur only when the nearest-neighbor Coulomb repulsion is sufficiently strong; 2) a spin-Peierls state can coexist with the ..1010..CO; and 3) experimental evidence clearly supports ..1100.. CO in the (TMTSF) and the 1:2 anionic CTS, while in the (TMTTF) salts the nature of the order is not yet clear.
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页码:681 / 682
页数:2
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