Future of nano-/hierarchical zeolites in catalysis: gaseous phase or liquid phase system

被引：87
|
作者：
Yan, Yueer [1 ]
Guo, Xiao [1 ]
Zhang, Yahong [1 ]
Tang, Yi [1 ]
机构：
[1] Fudan Univ, Dept Chem, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China
来源：
CATALYSIS SCIENCE & TECHNOLOGY | 2015年 / 5卷 / 02期
关键词：
NANOCRYSTALLINE ZSM-5 ZEOLITE; MESOPOROUS MOLECULAR-SIEVES; FRIEDEL-CRAFTS ACYLATION; TI-BETA CATALYST; H-BEA ZEOLITE; HIERARCHICAL ZEOLITES; ACETIC-ANHYDRIDE; MFI ZEOLITE; HYDROTHERMAL SYNTHESIS; HYDROGEN-PEROXIDE;
D O I：
10.1039/c4cy01114g
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Nano-/hierarchical zeolites have received increasing attention due to their catalytic performance preferable to that of conventional zeolites. The two major textural features of nano-/hierarchical zeolites, i.e. short microporous channel and large external surface area, can provide them with high activity and lifetime as well as high selectivity for products during catalysis. This perspective focuses on the most representative behavior of nano-/hierarchical zeolites in gaseous phase and liquid phase catalytic systems, considering whether the reaction is predominantly catalyzed within the micropore or at the external surface, and whether it is shape-selective. The catalytic characteristics and future prospects of nano-/hierarchical zeolites are highlighted in their applications in gaseous and liquid phase reactions.
引用
收藏
页码：772 / 785
页数：14
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