Significant magneto-elastic coupling at Griffiths-like phase boundaries in low dimensional oxides, ASb2O6 (A = Ni and Mn)

被引:2
|
作者
Chatterjee, A. [1 ]
Indra, A. [1 ,2 ]
Gutowski, O. [3 ]
von Zimmerman, M. [3 ]
Majumdar, S. [1 ]
Giri, S. [1 ]
机构
[1] Indian Assoc Cultivat Sci, Sch Phys Sci, Kolkata 700032, India
[2] Sri Krishna Coll, Dept Phys, Nadia 741502, WB, India
[3] DESY, Notkestr 85, D-22607 Hamburg, Germany
关键词
magneto-elastic effects; Griffiths phase; magnetic properties; SHORT-RANGE; CRYSTAL-STRUCTURE; TRANSITION; BEHAVIOR; GROWTH; ORDER;
D O I
10.1088/1361-648X/abe350
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The compounds, NiSb2O6 (NSO) and MnSb2O6 (MSO) attract the community for the quasi one-dimensional and layered structure composed of Ni2+ and Mn2+, which orders antiferromagnetically at T (N) = 6.7 and 12 K, respectively. Here, we report the Griffiths-like phase much above T (N) in the range of 37-85 K and 25-80 K for NSO and MSO, respectively. The dc magnetization results indicate the Griffiths-like phase, following the modified Curie-Weiss law. The magneto-capacitive responses for both the compounds show anomalies at the onset of the Griffiths-like phase. Intriguingly, the low temperature synchrotron diffraction results are conclusive for determining the singularities for both the compounds. Interplay between the low-dimensionality, magnetic frustration, and magneto-elastic coupling correlates the observed short range ordered state, which is suggested as a Griffiths-like phase, above T (N) for both the compounds.
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页数:9
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