Syntheses of C33-, C35-, and C39-Peridinin and Their Spectral Characteristics

被引：17

作者：

Kajikawa, Takayuki ^{[1
]}

Hasegawa, Shinji ^{[1
]}

Iwashita, Takashi ^{[2
]}

Kusumoto, Toshiyuki ^{[3
,4
]}

Hashimoto, Hideki ^{[3
,4
]}

Niedzwiedzki, Dariusz M. ^{[5
]}

Frank, Harry A. ^{[5
]}

Katsumura, Shigeo ^{[1
]}

机构：

[1] Kwansei Gakuin Univ, Dept Chem, Sch Sci & Technol, Sanda, Hyogo 6691337, Japan

[2] Suntory Inst Bioorgan Res, Osaka 6188503, Japan

[3] Osaka City Univ, Grad Sch Sci, Dept Phys, Sumiyoshi Ku, Osaka 5588585, Japan

[4] Osaka City Univ, Grad Sch Sci, CREST JST, Sumiyoshi Ku, Osaka 5588585, Japan

[5] Univ Connecticut, Dept Chem, Storrs, CT 06269 USA

来源：

ORGANIC LETTERS | 2009年 / 11卷 / 21期

基金：

美国国家卫生研究院;

关键词：

STEREOCONTROLLED TOTAL-SYNTHESIS; CARBONYL-COMPOUNDS; ALGAL CAROTENOIDS; PERIDININ; PROTEIN; COMPLEX; LIFETIME; BEHAVIOR;

D O I：

10.1021/ol901940g

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

Peridinin, a nor-carotenoid, exhibits an exceptionally high energy transfer efficiency to chlorophyll a in photosynthesis in the sea. This efficiency would be related to the unique structure of peridinin. To answer the question of why peridinin possesses the irregular C37 skeleton, we have achieved the synthesis of three peridinin derivatives. Their ultrafast time-resolved optical absorption and Stark spectra measurements have shown the presence of the characteristic intramolecular charge transfer state and the featured electrostatic properties of peridinin.

引用

页码：5006 / 5009

页数：4

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