Dynamically tuned non-classical light emission from atomic defects in hexagonal boron nitride

被引:40
|
作者
Lazic, Snezana [1 ,2 ]
Espinha, Andre [1 ,2 ]
Yanguas, Sergio Pinilla [1 ,2 ]
Gibaja, Carlos [3 ,4 ]
Zamora, Felix [3 ,4 ]
Ares, Pablo [4 ,5 ]
Chhowalla, Manish [6 ]
Paz, Wendel S. [7 ]
Palacios Burgos, Juan Jose [4 ,5 ]
Hernandez-Minguez, Alberto [8 ]
Santos, Paulo V. [8 ]
van der Meulen, Herko P. [1 ,2 ]
机构
[1] Univ Autonoma Madrid, Inst Univ Ciencia Mat Nicolas Cabrera INC, Dept Fis Mat, E-28049 Madrid, Spain
[2] Univ Autonoma Madrid, Condensed Matter Phys Ctr IFIMAC, E-28049 Madrid, Spain
[3] Univ Autonoma Madrid, Dept Quim Inorgan, E-28049 Madrid, Spain
[4] Univ Autonoma Madrid, IFIMAC, E-28049 Madrid, Spain
[5] Univ Autonoma Madrid, INC, Dept Fis Mat Condensada, E-28049 Madrid, Spain
[6] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England
[7] Univ Fed Rio De Janeiro, Inst Fis, Caixa Postal 68528, BR-21941972 Rio De Janeiro, RJ, Brazil
[8] Leibniz Inst Forsch Verbund Berlin eV, Paul Drude Inst Festkorperelektron, Hausvogteipl 5-7, D-10117 Berlin, Germany
关键词
SINGLE-PHOTON EMITTERS; QUANTUM EMITTERS; POINT-DEFECTS; MODULATION;
D O I
10.1038/s42005-019-0217-6
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Luminescent defects in hexagonal boron nitride (h-BN) have recently emerged as a promising platform for non-classical light emission. On-chip solutions, however, require techniques for controllable in-situ manipulation of quantum light. Here, we demonstrate the dynamic spectral and temporal tuning of the optical emission from h-BN via moving acoustomechanical modulation induced by stimulated phonons. When perturbed by the propagating acoustic phonon, the optically probed radiative h-BN defects are periodically strained and their sharp emission lines are modulated by the deformation potential coupling. This results in an acoustically driven spectral tuning within a 2.5-meV bandwidth. Our findings, supported by first-principles theoretical calculations, reveal exceptionally high elasto-optic coupling in hBN of -50 meV/%. Temporal control of the emitted photons is achieved by combining the acoustically mediated fine-spectral tuning with spectral detection filtering. This study opens the door to the use of sound for scalable integration of h-BN emitters in nanophotonic and quantum information technologies.
引用
收藏
页数:8
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