Synthesis and performance analysis of a mesoporous polydopamine-functionalized magnetic microcapsule adsorbent in water treatment

被引:6
|
作者
Zhou, Gang
Jiang, Wenjing
Xu, Zhuo
Yang, Siao
Jia, Xianchao
Tian, Yichun
Luan, Guoliang
机构
[1] Shandong Univ Sci & Technol, Coll Safety & Environm Engn, Qingdao 266590, Peoples R China
[2] Shandong Univ Sci & Technol, State Key Lab Min Disaster Prevent & Control, Shandong Prov & Minist Sci & Technol, Qingdao 266590, Peoples R China
基金
中国国家自然科学基金;
关键词
MagneticFe(3)O(4); Polydopamine; Nano-SiO2; Adsorption; Multifunctional material; SELECTIVE ADSORPTION; HIGHLY-EFFICIENT; AQUEOUS-SOLUTION; METHYLENE-BLUE; DYE; REMOVAL; RECYCLABILITY; NANOPARTICLES; KINETICS; CADMIUM;
D O I
10.1016/j.jwpe.2022.102894
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To scientifically and effectively solve the environmental and human hazards of polluted water bodies, this study uses the superparamagnetism of Fe3O4, the biocompatibility of mussel biomimetic polydopamine, and the large specific surface area and pore volume of mesoporous materials. Layer-by-layer self-assembled aminofunctionalized modified nano-SiO2 particles were used to prepare mesoporous PDA-functionalized magnetic microcapsule adsorbents (FMNAs). After a series of microscopic characterization and performance measurement experiments, it can be concluded that the relatively large surface area (55.844m(2)/g) and pore volume (0.438 cm3/g) in the mesoporous structure of FMNAs provide a large number of active adsorption sites and exhibit high adsorption capacity for MB, AF and Cd (II), which are 42.35, 46.20 and 40.70 mg/g, respectively. The adsorption process of FMANs is mainly controlled by chemical adsorption, which conforms to Langmuir and Freundlich isothermal model, superparamagnetism gives FMNAs good repeatability.
引用
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页数:11
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