Metal-organic frameworks (ZIF-67) as efficient cocatalysts for photocatalytic reduction of CO2: the role of the morphology effect

被引：243

作者：

Wang, Mang ^{[1
]}

Liu, Jinxuan ^{[1
]}

Guo, Chunmei ^{[1
]}

Gao, Xiaosu ^{[1
]}

Gong, Chenghuan ^{[1
]}

Wang, Yan ^{[2
]}

Liu, Bo ^{[2
]}

Li, Xiaoxin ^{[1
]}

Gurzadyan, Gagik G. ^{[1
]}

Sun, Licheng ^{[1
,3
]}

机构：

[1] Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China

[2] Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China

[3] KTH Royal Inst Technol, Dept Chem, S-110044 Stockholm, Sweden

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2018年 / 6卷 / 11期

关键词：

ZEOLITIC IMIDAZOLATE FRAMEWORK; CARBON-DIOXIDE; VISIBLE-LIGHT; CATALYSTS; CHALLENGES; CONVERSION; CAPTURE; FUELS; STATE;

D O I：

10.1039/c8ta00154e

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Metal-organic frameworks (MOFs), ZIF-67, with different morphologies were synthesized via a solvent-induced method at room temperature. The photocatalytic performances towards the reduction of CO2 were evaluated by using ZIF-67 materials as cocatalysts cooperating with a ruthenium-based complex as the photosensitizer. It has been demonstrated that the two-dimensional ZIF-67 with a leaf-like morphology exhibited the best photocatalytic activity and stability due to the highest CO2 adsorption capability and efficient electron transfer from the excited [Ru(bpy)(3)](2+) to ZIF-67.

引用

页码：4768 / 4775

页数：8

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