Spin liquid state in κ-(BEDT-TTF)2Cu2(CN)3 studied by muon spin relaxation method

被引:0
|
作者
Ohira, S. [1 ]
Shimizu, Y.
Kanoda, K.
Saito, G.
机构
[1] RIKEN, Adv Meson Sci Lab, Wako, Saitama 3510198, Japan
[2] RIKEN, Condensed Mol Mat Lab, Wako, Saitama 3510198, Japan
[3] Univ Tokyo, CREST, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan
[4] Kyoto Univ, Div Chem, Sakyo Ku, Kyoto 6068502, Japan
关键词
D O I
10.1007/BF02679485
中图分类号
O59 [应用物理学];
学科分类号
摘要
Magnetic Properties of an organic Mott insulator with an approximately isotropic. triangular lattice structure, kappa-(ET)(2)Cu-2(CN)(3), are investigated by the muon spin relaxation (mu SR) method. No magnetic ordering is observed down to 20 mK in the zero-field (ZF) mu SR measurement, suggesting the realization of the spin liquid ground state. An enhancement of the distribution of internal fields, corresponding to broadening of the linewidth reported in the C-13 NMR study under magnetic fields, is not observed under ZF. A slight change in the spin dynamics is detected below 4 K. This change is quite small and different from the critical slow-down effect attributable to a magnetic transition.
引用
收藏
页码:153 / 158
页数:6
相关论文
共 50 条
  • [1] Spin liquid state inκ-(BEDT-TTF)2Cu2(CN)3 studied by muon spin relaxation method
    S. Ohira
    Y. Shimizu
    K. Kanoda
    G. Saito
    [J]. Journal of Low Temperature Physics, 2006, 142 : 153 - 158
  • [2] Spin Liquid State in κ-(BEDT-TTF)2Cu2(CN)3 Studied by Muon Spin Relaxation Method
    S. Ohira
    Y. Shimizu
    K. Kanoda
    G. Saito
    [J]. Journal of Low Temperature Physics, 2006, 142 : 153 - 158
  • [3] (BEDT-TTF)2Cu2(CN)3 Spin Liquid: Beyond the Average Structure
    Foury-Leylekian, Pascale
    Ilakovac-Casses, Vita
    Baledent, Victor
    Fertey, Pierre
    Arakcheeva, Alla
    Milat, Ognjen
    Petermann, Denis
    Guillier, Gilles
    Miyagawa, Kazuya
    Kanoda, Kazushi
    Alemany, Pere
    Canadell, Enric
    Tomic, Silvia
    Pouget, Jean-Paul
    [J]. CRYSTALS, 2018, 8 (04):
  • [4] Gapped magnetic ground state in quantum spin liquid candidate κ-(BEDT-TTF)2Cu2(CN)3
    Miksch, Bjorn
    Pustogow, Andrej
    Rahim, Mojtaba Javaheri
    Bardin, Andrey A.
    Kanoda, Kazushi
    Schlueter, John A.
    Hubner, Ralph
    Scheffler, Marc
    Dressel, Martin
    [J]. SCIENCE, 2021, 372 (6539) : 276 - +
  • [5] Quantum criticality in an organic spin-liquid insulator κ-(BEDT-TTF)2Cu2(CN)3
    Isono, Takayuki
    Terashima, Taichi
    Miyagawa, Kazuya
    Kanoda, Kazushi
    Uji, Shinya
    [J]. NATURE COMMUNICATIONS, 2016, 7
  • [6] Microscopic Phase Separation in Triangular-Lattice Quantum Spin Magnet κ-(BEDT-TTF)2Cu2(CN)3 Probed by Muon Spin Relaxation
    Nakajima, Saori
    Suzuki, Takao
    Ishii, Yasuyuki
    Ohishi, Kazuki
    Watanabe, Isao
    Goto, Takayuki
    Oosawa, Akira
    Yoneyama, Naoki
    Kobayashi, Norio
    Pratt, Francis L.
    Sasaki, Takahiko
    [J]. JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2012, 81 (06)
  • [7] Quantum criticality in an organic spin-liquid insulator κ-(BEDT-TTF)2Cu2(CN)3
    Takayuki Isono
    Taichi Terashima
    Kazuya Miyagawa
    Kazushi Kanoda
    Shinya Uji
    [J]. Nature Communications, 7
  • [8] Anisotropic charge dynamics in the quantum spin-liquid candidate κ-(BEDT-TTF)2Cu2(CN)3
    Pinteric, M.
    Culo, M.
    Milat, O.
    Basletic, M.
    Korin-Hamzic, B.
    Tafra, E.
    Hamzic, A.
    Ivek, T.
    Peterseim, T.
    Miyagawa, K.
    Kanoda, K.
    Schlueter, J. A.
    Dressel, M.
    Tomic, S.
    [J]. PHYSICAL REVIEW B, 2014, 90 (19)
  • [9] Magnetodielectric effects and spin-charge coupling in the spin-liquid candidate κ-(BEDT-TTF)2Cu2(CN)3
    Poirier, Mario
    Parent, Samuel
    Cote, Alex
    Miyagawa, Kazuya
    Kanoda, Kazushi
    Shimizu, Yasuhiro
    [J]. PHYSICAL REVIEW B, 2012, 85 (13)
  • [10] Thirty-Year Anniversary of κ-(BEDT-TTF)2Cu2(CN)3: Reconciling the Spin Gap in a Spin-Liquid Candidate
    Pustogow, Andrej
    [J]. SOLIDS, 2022, 3 (01): : 93 - 110