Perylene Diimide Based Imine Cages for Inclusion of Aromatic Guest Molecules and Visible-Light Photocatalysis

被引：19

作者：

Feng, Xiying ^{[1
]}

Liao, Peisen ^{[1
]}

Jiang, Jingxing ^{[1
]}

Shi, Jianying ^{[1
]}

Ke, Zhuofeng ^{[1
]}

Zhang, Jianyong ^{[1
]}

机构：

[1] Sun Yat Sen Univ, MOE Lab Polymer Composite & Funct Mat, Sch Mat Sci & Engn, Guangzhou 510275, Guangdong, Peoples R China

来源：

CHEMPHOTOCHEM | 2019年 / 3卷 / 10期

关键词：

chirality; host-guest systems; organic cages; perylene diimide; photocatalysis; supramolecular chemistry; POROUS ORGANIC CAGE; PALLADIUM NANOPARTICLES EFFICIENT; HETEROGENEOUS CATALYSTS; ELECTRON; COMPLEXATION; FLUORESCENCE; MACROCYCLES; SEPARATION; VERTICES; AFFINITY;

D O I：

10.1002/cptc.201900058

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A strategy for the development of visible-light-sensitive organic cage structures is reported. Enantiomeric imine cages with optical and electrochemical properties are developed employing perylene diimide (PDI) and tetraphenylethene subunits using dynamic covalent imine chemistry. Polycyclic aromatic hydrocarbons are encapsulated efficiently in the imine cage, and the guests interact with PDI units via supramolecular pi-pi interactions. Visible-light-driven Smiles rearrangement of 2-aryloxybenzoic acids to aryl salicylates is achieved with high efficiency in the presence of the imine cage as the catalyst.

引用

页码：1014 / 1019

页数：6

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