Self-forming double-crosslinked hydrogels by the marriage of catechols and enzyme mimetic polymers

被引：1

作者：

Chen, Yaqing ^{[1
,2
]}

Misselwitz, Erik ^{[1
,2
]}

Agergaard, Asger Holm ^{[1
,2
]}

Andersen, Amanda ^{[1
,2
]}

Pedersen, Carsten ^{[1
,2
]}

Birkedal, Henrik ^{[1
,2
]}

机构：

[1] Aarhus Univ, Dept Chem, Gustav Wieds Vej 14, DK-8000 Aarhus, Denmark

[2] Aarhus Univ, Interdisciplinary Nanosci Ctr iNANO, Gustav Wieds Vej 14, DK-8000 Aarhus, Denmark

来源：

CHEMICAL COMMUNICATIONS | 2022年 / 58卷 / 45期

关键词：

MUSSEL; LINKING; PROTEIN; NEREIS; ZINC; COPPER(II); TYROSINASE; MIMICKING; COMPLEXES; MECHANICS;

D O I：

10.1039/d2cc01290a

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Self-forming double-crosslinked (DC) hydrogels were designed by incorporating enzyme-mimicking metal coordination polymer crosslinks and catechol chemistry. A macromolecular tris-histidine copper complex acted both as part of the hydrogel network and as a catalyst of catechol oxidation to induce a second hydrogel network by covalent crosslinking of catechol functionalized polymers thus giving catalytic control over hydrogel crosslinking.

引用

页码：6526 / 6529

页数：4

共 38 条

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