Nitrous oxide emissions 1999 to 2009 from a global atmospheric inversion

被引:50
|
作者
Thompson, R. L. [1 ]
Chevallier, F. [2 ]
Crotwell, A. M. [3 ,11 ]
Dutton, G. [3 ]
Langenfelds, R. L. [4 ]
Prinn, R. G. [5 ]
Weiss, R. F. [6 ]
Tohjima, Y. [7 ]
Nakazawa, T. [8 ]
Krummel, P. B. [4 ]
Steele, L. P. [4 ]
Fraser, P. [4 ]
O'Doherty, S. [9 ]
Ishijima, K. [10 ]
Aoki, S. [9 ]
机构
[1] Norwegian Inst Air Res, Kjeller, Norway
[2] Lab Sci Climat & Environm, Gif Sur Yvette, France
[3] NOAA, ESRL, Global Monitoring Div, Boulder, CO USA
[4] Commonwealth Sci & Ind Res Org, Aspendale, Vic, Australia
[5] MIT, Ctr Global Change Sci, Cambridge, MA 02139 USA
[6] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA
[7] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan
[8] Tohoku Univ, Ctr Atmospher & Ocean Studies, Grad Sch Sci, Sendai, Miyagi 9808578, Japan
[9] Univ Bristol, Sch Chem, Atmospher Chem Res Grp, Bristol, Avon, England
[10] Japan Agcy Marine Earth Sci & Technol, Yokohama, Kanagawa, Japan
[11] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
关键词
N2O; CO2; PERFORMANCE; LIFETIMES; HISTORY; FLUXES; SCHEME; OCEANS; MODEL; CYCLE;
D O I
10.5194/acp-14-1801-2014
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
N2O surface fluxes were estimated for 1999 to 2009 using a time-dependent Bayesian inversion technique. Observations were drawn from 5 different networks, incorporating 59 surface sites and a number of ship-based measurement series. To avoid biases in the inverted fluxes, the data were adjusted to a common scale and scale offsets were included in the optimization problem. The fluxes were calculated at the same resolution as the transport model (3.75 degrees longitude x 2.5 degrees latitude) and at monthly time resolution. Over the 11-year period, the global total N2O source varied from 17.5 to 20.1 Tg a(-1) N. Tropical and subtropical land regions were found to consistently have the highest N2O emissions, in particular in South Asia (20 +/- 3% of global total), South America (13 +/- 4 %) and Africa (19 +/- 3 %), while emissions from temperate regions were smaller: Europe (6 +/- 1 %) and North America (7 +/- 2 %). A significant multi-annual trend in N2O emissions (0.045 Tg a(-2) N) from South Asia was found and confirms inventory estimates of this trend. Considerable interannual variability in the global N2O source was observed (0.8 Tg a(-1) N, 1 standard deviation, SD) and was largely driven by variability in tropical and subtropical soil fluxes, in particular in South America (0.3 Tg a(-1) N, 1 SD) and Africa (0.3 Tg a(-1) N, 1 SD). Notable variability was also found for N2O fluxes in the tropical and southern oceans (0.15 and 0.2 Tg a(-1) N, 1 SD, respectively). Interannual variability in the N2O source shows some correlation with the El Nino-Southern Oscillation (ENSO), where El Nino conditions are associated with lower N2O fluxes from soils and from the ocean and vice versa for La Nina conditions.
引用
收藏
页码:1801 / 1817
页数:17
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