Modeling of hazardous air pollutant removal in the pulsed corona discharge

被引:15
|
作者
Derakhshesh, Marzie [1 ]
Abedi, Jalal [1 ]
Omidyeganeh, Mohammad [1 ]
机构
[1] Univ Calgary, Dept Chem & Petr Engn, Schulich Sch Engn, Calgary, AB T2N 1N4, Canada
基金
加拿大创新基金会;
关键词
VOLATILE ORGANIC-COMPOUNDS; NITRIC-OXIDE; REACTOR; DESTRUCTION; NITROGEN; KINETICS; SULFUR; N2O; NO;
D O I
10.1016/j.physleta.2009.01.041
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
This study investigated the effects of two parts of the performance equation of the pulsed corona reactor, which is one of the non-thermal plasma processing tools of atmospheric pressure for eliminating pollutant streams. First, the effect of axial dispersion in the diffusion term and then the effect of different orders of the reaction in the decomposition rate term were considered. The mathematical model was primarily developed to predict the effluent concentration of the pulsed corona reactor using mass balance, and considering axial dispersion, linear velocity and decomposition rate of pollutant. The steady state form of this equation was subsequently solved assuming different reaction orders. For the derivation of the performance equation of the reactor, it was assumed that the decomposition rate of the pollutant was directly proportional to discharge power and the concentration of the pollutant. The results were validated and compared with another predicted model using their experimental data. The model developed in this study was also validated with two other experimental data in the literature for N2O. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:1051 / 1057
页数:7
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